Organic Photovoltaics Utilizing Small-Molecule Donors and Y-Series Nonfullerene Acceptors

被引：43
作者：
Ge, Jinfeng [1 ,2 ]
Xie, Lin [1 ]
Peng, Ruixiang [1 ,2 ]
Ge, Ziyi [1 ,2 ]
机构：
[1] Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Peoples R China
[2] Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, Beijing 100049, Peoples R China
来源：
ADVANCED MATERIALS | 2023年 / 35卷 / 20期
基金：
中国国家自然科学基金;
关键词：
all-small-molecule organic solar cells; nonfullerene acceptors; POLYMER SOLAR-CELLS; BULK-HETEROJUNCTION BLENDS; 14-PERCENT EFFICIENCY; ELECTRON-ACCEPTOR; CONJUGATED POLYMER; LENGTH-SCALE; MORPHOLOGY; BENZODITHIOPHENE; PERFORMANCE; DESIGN;
D O I：
10.1002/adma.202206566
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
The emerging Y-series nonfullerene acceptors (Y-NFA) has prompted the rapid progress of power conversion efficiency (PCE) of all-small-molecule organic solar cells (ASM-OSCs) from around 12% to 17%. The excellent PCE improvement benefits from not only the outstanding properties of Y-series acceptors but also the successful development of small-molecule donors. The short-circuit current density, fill factor, and nonradiative recombination are all optimized to the unprecedented values, providing a scenery that is obviously different from the ITIC-series based ASM-OSCs. In this review, OSCs utilizing small-molecule donors and Y-NFA are summarized and classified in order to provide an up-to-date development overview and give an insight on structure-property correlation. Then, the characteristics of bulk-heterojunction (BHJ) formation of ASM-OSCs are discussed and compared with that of polymer-based OSCs. Finally, the challenges and outlook on designing ground-breaking small-molecule donor and forming an ideal BHJ morphology are discussed.
引用
收藏
页数：19
相关论文
共 131 条
[11]   A Chlorinated π-Conjugated Polymer Donor for Efficient Organic Solar Cells [J].
Chen, Hui ;
Hu, Zhiming ;
Wang, Huan ;
Liu, Longzhu ;
Chao, Pengjie ;
Qu, Jianfei ;
Chen, Wei ;
Liu, Anhua ;
He, Feng .
JOULE, 2018, 2 (08) :1623-1634
[12]   Molecular ordering and phase segregation induced by a volatile solid additive for highly efficient all-small-molecule organic solar cells [J].
Chen, Shanshan ;
Ye, Junfeng ;
Yang, Qianguang ;
Oh, Jiyeon ;
Hu, Dingqin ;
Yang, Ke ;
Odunmbaku, George Omololu ;
Li, Feng ;
Yu, Qingqing ;
Kan, Zhipeng ;
Xiao, Zeyun ;
Yang, Changduk ;
Lu, Shirong ;
Sun, Kuan .
JOURNAL OF MATERIALS CHEMISTRY A, 2021, 9 (05) :2857-2863
[13]   Realizing 19.05% Efficiency Polymer Solar Cells by Progressively Improving Charge Extraction and Suppressing Charge Recombination [J].
Chong, Kaien ;
Xu, Xiaopeng ;
Meng, Huifeng ;
Xue, Jingwei ;
Yu, Liyang ;
Ma, Wei ;
Peng, Qiang .
ADVANCED MATERIALS, 2022, 34 (13)
[14]   Small is Powerful: Recent Progress in Solution-Processed Small Molecule Solar Cells [J].
Collins, Samuel D. ;
Ran, Niva A. ;
Heiber, Michael C. ;
Thuc-Quyen Nguyen .
ADVANCED ENERGY MATERIALS, 2017, 7 (10)
[15]   Single-Junction Organic Photovoltaic Cells with Approaching 18% Efficiency [J].
Cui, Yong ;
Yao, Huifeng ;
Zhang, Jianqi ;
Xian, Kaihu ;
Zhang, Tao ;
Hong, Ling ;
Wang, Yuming ;
Xu, Ye ;
Ma, Kangqiao ;
An, Cunbin ;
He, Chang ;
Wei, Zhixiang ;
Gao, Feng ;
Hou, Jianhui .
ADVANCED MATERIALS, 2020, 32 (19)
[16]   Achieving Over 15% Efficiency in Organic Photovoltaic Cells via Copolymer Design [J].
Cui, Yong ;
Yao, Huifeng ;
Hong, Ling ;
Zhang, Tao ;
Xu, Ye ;
Xian, Kaihu ;
Gao, Bowei ;
Qin, Jinzhao ;
Zhang, Jianqi ;
Wei, Zhixiang ;
Hou, Jianhui .
ADVANCED MATERIALS, 2019, 31 (14)
[17]   Fluorination-enabled optimal morphology leads to over 11% efficiency for inverted small-molecule organic solar cells [J].
Deng, Dan ;
Zhang, Yajie ;
Zhang, Jianqi ;
Wang, Zaiyu ;
Zhu, Lingyun ;
Fang, Jin ;
Xia, Benzheng ;
Wang, Zhen ;
Lu, Kun ;
Ma, Wei ;
Wei, Zhixiang .
NATURE COMMUNICATIONS, 2016, 7
[18]   Improving Molecular Planarity by Changing Alky Chain Position Enables 12.3% Efficiency All-Small-Molecule Organic Solar Cells with Enhanced Carrier Lifetime and Reduced Recombination [J].
Dong, Xiyue ;
Yang, Ke ;
Tang, Hua ;
Hu, Dingqin ;
Chen, Shanshan ;
Zhang, Jun ;
Kan, Zhipeng ;
Duan, Tainan ;
Hu, Chao ;
Dai, Xuexin ;
Xiao, Zeyun ;
Sun, Kuan ;
Lu, Shirong .
SOLAR RRL, 2020, 4 (01)
[19]   Systematic Investigation of Benzodithiophene- and Diketopyrrolopyrrole-Based Low-Bandgap Polymers Designed for Single Junction and Tandem Polymer Solar Cells [J].
Dou, Letian ;
Gao, Jing ;
Richard, Eric ;
You, Jingbi ;
Chen, Chun-Chao ;
Cha, Kitty C. ;
He, Youjun ;
Li, Gang ;
Yang, Yang .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2012, 134 (24) :10071-10079
[20]   Simple thiazole-centered oligothiophene donor enables 15.4% efficiency all small molecule organic solar cells [J].
Duan, Tainan ;
Chen, Qianqian ;
Yang, Qianguang ;
Hu, Dingqin ;
Cai, Guilong ;
Lu, Xinhui ;
Lv, Jie ;
Song, Hang ;
Zhong, Cheng ;
Liu, Feng ;
Yu, Donghong ;
Lu, Shirong .
JOURNAL OF MATERIALS CHEMISTRY A, 2022, 10 (06) :3009-3017
12345678910