Recent advances in supramolecular fullerene chemistry

被引:77
作者
Chang, Xingmao [1 ,2 ]
Xu, Youzhi [1 ]
von Delius, Max [2 ]
机构
[1] Henan Univ, Coll Chem & Mol Sci, Kaifeng 475004, Peoples R China
[2] Ulm Univ, Inst Organ Chem, D-89081 Ulm, Germany
基金
美国国家科学基金会;
关键词
REGIOSELECTIVE BIS-FUNCTIONALIZATION; PHOTOINDUCED ELECTRON-TRANSFER; DYNAMIC COVALENT CHEMISTRY; METAL-ORGANIC FRAMEWORKS; FIELD-EFFECT TRANSISTORS; HOST-GUEST INTERACTIONS; CHARGE-SEPARATED STATE; MOLECULAR RECOGNITION; PHOTOPHYSICAL PROPERTIES; SELECTIVE COMPLEXATION;
D O I
10.1039/d2cs00937d
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Fullerene chemistry has come a long way since 1990, when the first bulk production of C-60 was reported. In the past decade, progress in supramolecular chemistry has opened some remarkable and previously unexpected opportunities regarding the selective (multiple) functionalization of fullerenes and their (self)assembly into larger structures and frameworks. The purpose of this review article is to provide a comprehensive overview of these recent developments. We describe how macrocycles and cages that bind strongly to C-60 can be used to block undesired addition patterns and thus allow the selective preparation of single-isomer addition products. We also discuss how the emergence of highly shape-persistent macrocycles has opened opportunities for the study of photoactive fullerene dyads and triads as well as the preparation of mechanically interlocked compounds. The preparation of two- or three-dimensional fullerene materials is another research area that has seen remarkable progress over the past few years. Due to the rapidly decreasing price of C-60 and C-70, we believe that these achievements will translate into all fields where fullerenes have traditionally (third-generation solar cells) and more recently been applied (catalysis, spintronics).
引用
收藏
页码:47 / 83
页数:38
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