Role of molecular alignment in attosecond photoionization of N2

被引：4

作者：

Zhang, Ru ^{[1
]}

Wang, Feng ^{[1
]}

Liao, Qing ^{[1
]}

Lu, Peixiang ^{[1
,2
]}

机构：

[1] Wuhan Inst Technol, Hubei Key Lab Opt Informat & Pattern Recognit, Wuhan 430205, Peoples R China

[2] Guangdong Intelligent Robot Inst, Dongguan 523808, Peoples R China

来源：

PHYSICAL REVIEW A | 2023年 / 108卷 / 01期

基金：

中国国家自然科学基金;

关键词：

TIME; DELAY; DEPENDENCE;

D O I：

10.1103/PhysRevA.108.013113

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

We theoretically study the influence of molecular alignment on the attosecond photoionization of the N-2 molecule. Based on the numerical simulations of the single-active-electron two-dimensional time-dependent Schrodinger equation, we find that the alignment-averaged photoelectron momentum distributions deviate from the single-molecule result, especially for a large molecular alignment angle and a low degree of molecular alignment. As a result, the photoemission time delays extracted from the angular-averaged streaking spectra are different from the single-molecule result. More importantly, the alignment-averaged photoemission time delays are found to depend on the degree of molecular alignment as well as the molecular alignment distribution. Our results reveal the important role of molecular alignment in the molecular attosecond photoionization.

引用

页数：8

共 43 条

[1] Polarization Effects in Attosecond Photoelectron Spectroscopy [J].

Baggesen, Jan Conrad ;

Madsen, Lars Bojer .

PHYSICAL REVIEW LETTERS, 2010, 104 (04)

[2] Theory of attosecond delays in molecular photoionization [J].

Baykusheva, Denitsa ;

Woerner, Hans Jakob .

JOURNAL OF CHEMICAL PHYSICS, 2017, 146 (12) :124306

[3] Attosecond-resolved photoionization of chiral molecules [J].

Beaulieu, S. ;

Comby, A. ;

Clergerie, A. ;

Caillat, J. ;

Descamps, D. ;

Dudovich, N. ;

Fabre, B. ;

Geneaux, R. ;

Legare, F. ;

Petit, S. ;

Pons, B. ;

Porat, G. ;

Ruchon, T. ;

Taieb, R. ;

Blanchet, V. ;

Mairesse, Y. .

SCIENCE, 2017, 358 (6368) :1288-1293

[4] Attosecond Resolved Electron Release in Two-Color Near-Threshold Photoionization of N2 [J].

Caillat, Jeremie ;

Maquet, Alfred ;

Haessler, Stefan ;

Fabre, Baptiste ;

Ruchon, Thierry ;

Salieres, Pascal ;

Mairesse, Yann ;

Taieb, Richard .

PHYSICAL REVIEW LETTERS, 2011, 106 (09)

[5] Attosecond delay in the molecular photoionization of asymmetric molecules [J].

Chacon, Alexis ;

Ruiz, Camilo .

OPTICS EXPRESS, 2018, 26 (04) :4548-4562

[6] Anisotropic photoemission time delays close to a Fano resonance [J].

Cirelli, Claudio ;

Marante, Carlos ;

Heuser, Sebastian ;

Petersson, C. L. M. ;

Jimenez Galan, Alvaro ;

Argenti, Luca ;

Zhong, Shiyang ;

Busto, David ;

Isinger, Marcus ;

Nandi, Saikat ;

Maclot, Sylvain ;

Rading, Linnea ;

Johnsson, Per ;

Gisselbrecht, Mathieu ;

Lucchini, Matteo ;

Gallmann, Lukas ;

Dahlstrom, J. Marcus ;

Lindroth, Eva ;

L'Huillier, Anne ;

Martin, Fernando ;

Keller, Ursula .

NATURE COMMUNICATIONS, 2018, 9

[7] INTERFERENCE IN PHOTO-IONIZATION OF MOLECULES [J].

COHEN, HD ;

FANO, U .

PHYSICAL REVIEW, 1966, 150 (01) :30-&

[8] Methods for the measurement of the duration of high-harmonic pulses [J].

Constant, E ;

Taranukhin, VD ;

Stolow, A ;

Corkum, PB .

PHYSICAL REVIEW A, 1997, 56 (05) :3870-3878

[9] APPLICATION OF THE IMAGINARY TIME STEP METHOD TO THE SOLUTION OF THE STATIC HARTREE-FOCK PROBLEM [J].

DAVIES, KTR ;

FLOCARD, H ;

KRIEGER, S ;

WEISS, MS .

NUCLEAR PHYSICS A, 1980, 342 (01) :111-123

[10] X-ray pulses approaching the attosecond frontier [J].

Drescher, M ;

Hentschel, M ;

Kienberger, R ;

Tempea, G ;

Spielmann, C ;

Reider, GA ;

Corkum, PB ;

Krausz, F .

SCIENCE, 2001, 291 (5510) :1923-1927

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