Treatment of Mixture Pollutants with Combined Plasma Photocatalysis in Continuous Tubular Reactors with Atmospheric-Pressure Environment: Understanding Synergetic Effect Sources

被引:5
|
作者
Khezami, Lotfi [1 ]
Assadi, Aymen Amin [2 ,3 ]
机构
[1] Imam Mohammad Ibn Saud Islamic Univ IMSIU, Coll Sci, Dept Chem, POB 5701, Riyadh 11432, Saudi Arabia
[2] Imam Mohammad Ibn Saud Islamic Univ IMSIU, Coll Engn, POB 5701, Riyadh 11432, Saudi Arabia
[3] Univ Rennes, Ecole Natl Super Chim Rennes, ISCR Inst Sci Chim Rennes UMR 6226, CNRS, Campus Beaulieu,Av Gen Leclerc, F-35000 Rennes, France
关键词
mixture of pollutants; coupling system; plasma; photocatalysis; synergetic effect; mineralization; VOLATILE ORGANIC-COMPOUNDS; GAS STREAMS; INDOOR AIR; DEGRADATION; TOLUENE; OXIDATION; REMOVAL;
D O I
10.3390/ma16216857
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
This study investigates the pilot-scale combination of nonthermal plasma and photocatalysis for removing Toluene and dimethyl sulfur (DMDS), examining the influence of plasma energy and initial pollutant concentration on the performance and by-product formation in both pure compounds and mixtures. The results indicate a consistent 15% synergy effect, improving Toluene conversion rates compared to single systems. Ozone reduction and enhanced CO2 selectivity were observed when combining plasma and photocatalysis. This process effectively treats pollutant mixtures, even those containing sulfur compounds. Furthermore, tests confirm nonthermal plasma's in-situ regeneration of the photocatalytic surface, providing a constant synergy effect.
引用
收藏
页数:15
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