Photochromism of three complexes based on 1-(4-carboxybutyl)-4,4′-bipyridinium ligand

被引：2
作者：
Chen, Jiali [1 ]
Yang, Fengyi [1 ]
Wang, Junwen [1 ]
Liu, Jinjian [1 ]
机构：
[1] Shanxi Normal Univ, Key Lab Magnet Mol & Magnet Informat Mat, Minist Educ, Taiyuan 030032, Peoples R China
来源：
POLYHEDRON | 2024年 / 249卷
关键词：
1-(4-Carboxybutyl)-44 ' -bipyridinium bromide; (HCPbpyBr); Crystal structure; Photochromism; Luminescent property; Inkless and erasable printing; METAL-ORGANIC FRAMEWORK; GOOD ANION; ADSORPTION; POLYMERS;
D O I：
10.1016/j.poly.2023.116796
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
Based on the viologen ligand 1-(4-carboxybutyl)-4,4 '-bipyridinium bromide (HCPbpyBr), three new complexes with different auxiliary ligands and metal ions have been prepared and structurally characterized, namely Ni(CPbpy)(H4BTEC)(0.5)(H2O)(4)<middle dot>(BTEC)(0.5)<middle dot>2H(2)O (1), Co(CPbpy)(H4BTEC)(0.5)(H2O)(4)<middle dot>(BTEC)(0.5)<middle dot>2H(2)O (2) and [Cd(CPbpy)(m-BDC)<middle dot>2H(2)O](n) (3) (1,2,4,5-benzenetetracarboxylic acid = H4BTEC, 1,3-benzenedicarboxylic acid = m-H2BDC). Complexes 1 and 2 have identical isolated structure, while complex 3 features a three-dimensional (3D) framework. Meanwhile, complex 3 exhibits electron-transfer (ET) UV and X-ray dual photochromism and photo-controlled luminescent properties, while photochromism is not observed in complexes 1 and 2. Additionally, complex 3 has the prospective application as an inkless and erasable printing material because of its excellent photochromic property.
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页数：7
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