Materials design and preparation for high energy density and high power density electrochemical supercapacitors

被引:150
作者
Dong, Wujie [1 ]
Xie, Miao [1 ]
Zhao, Siwei [2 ]
Qin, Qiuliang [1 ]
Huang, Fuqiang [1 ,2 ]
机构
[1] Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine M, Shanghai 200050, Peoples R China
[2] Peking Univ, Coll Chem & Mol Engn, State Key Lab Rare Earth Mat Chem & Applicat, Beijing 100871, Peoples R China
基金
中国国家自然科学基金;
关键词
supercapacitors; high energy density; high power density; electrochemical window; pseudocapacitance; HIGH-PERFORMANCE SUPERCAPACITOR; REDUCED GRAPHENE OXIDE; HIERARCHICAL POROUS CARBON; NITROGEN-DOPED CARBON; LITHIUM-ION BATTERIES; VANADIUM CARBIDE MXENE; VOLUMETRIC CAPACITIVE PERFORMANCE; TRANSITION-METAL DICHALCOGENIDE; ADVANCED ELECTRODE MATERIALS; SOLID-STATE SUPERCAPACITORS;
D O I
10.1016/j.mser.2022.100713
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Electrochemical supercapacitors process ultra-high power density and long lifetime, but the relatively low en-ergy density hinder the wide application. Therefore, supercapacitors with high energy density and high power density ("dual high") have attracted great attentions. New active materials with high pseudocapacitance beyond electronic double layer capacitance and novel devices with high working voltage, are two approaches toward "dual high" supercapacitors. In this review, we briefly introduce the history, classification, basic mechanism, and device architecture of supercapacitors. Then, the key issues and design strategies for "dual high" supercapacitors will be proposed. The recent methodical advances will also be highlighted on the material with outstanding specific capacitance and the corresponding electrolyte systems with expanded operating voltage. Besides, the recent progresses of current collectors and separators for supercapacitors are also included. Finally, we will provide our insights regarding the major challenges and prospective solutions in this highly exciting field. We believe such a review will significantly expand the horizons in ever-deepening understanding toward "dual high" supercapacitors
引用
收藏
页数:99
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