Synthesis, structure, and photocatalytic properties of a two-dimensional uranyl organic framework

被引：0

作者：

Meng, Yuning ^{[1
]}

Liu, Donghui ^{[1
]}

Lan, Qiaofa ^{[1
]}

Xie, Ziyu ^{[1
]}

Niu, Fei ^{[1
]}

Zhang, Xiaolin ^{[1
]}

Yang, Youming ^{[1
]}

机构：

[1] Jiangxi Univ Sci & Technol, Fac Mat Met & Chem, Ganzhou 341000, Peoples R China

来源：

ZEITSCHRIFT FUR KRISTALLOGRAPHIE-CRYSTALLINE MATERIALS | 2023年 / 238卷 / 1-2期

关键词：

methylene blue; photocatalytic; rhodamine B; uranyl organic framework; SPECTROSCOPY; COMPLEXES; FAMILY;

D O I：

10.1515/zkri-2022-0012

中图分类号：

O7 [晶体学];

学科分类号：

0702 ; 070205 ; 0703 ; 080501 ;

摘要：

A two-dimensional uranyl organic framework (UOF) UO2(L)(DMA) (1) (H2L = 2-aminoisophthalic acid, DMA = N, N-dimethylacetamide) has been solvothermally synthesized and characterized thoroughly by elemental analysis, infrared spectroscopy, single-crystal X-ray diffraction, solid fluorescence, powder X-ray diffraction, thermogravimetric analysis, and UV-visible spectroscopy. Furthermore, the degradation efficiencies of UOF 1 to organic dye methylene blue (MB) and rhodamine B (RhB) are 93.2 and 86.5% under irradiation of visible light which indicates that UOF 1 has remarkable photocatalytic activity. UOF 1 also displayed a certain selectivity for mixed dyes of MB & RhB.

引用

页码：65 / 71

页数：7

共 35 条

[1]

[Anonymous], 2015, SAINT

[2] Structural elucidation and physicochemical properties of mononuclear Uranyl(VI) complexes incorporating dianionic units [J].

Azam, Mohammad ;

Velmurugan, Gunasekaran ;

Wabaidur, Saikh Mohammad ;

Trzesowska-Kruszynska, Agata ;

Kruszynski, Rafal ;

Al-Resayes, Saud I. ;

Al-Othman, Zeid A. ;

Venuvanalingam, Ponnambalam .

SCIENTIFIC REPORTS, 2016, 6

[3] First Cationic Uranyl-Organic Framework with Anion-Exchange Capabilities [J].

Bai, Zhuanling ;

Wang, Yanlong ;

Li, Yuxiang ;

Liu, Wei ;

Chen, Lanhua ;

Sheng, Daopeng ;

Juan Diwu ;

Chai, Zhifang ;

Albrecht-Schmitt, Thomas E. ;

Wang, Shuao .

INORGANIC CHEMISTRY, 2016, 55 (13) :6358-6360

[4] Study of uranyl(VI) malonate complexation by time resolved laser-induced fluorescence spectroscopy (TRLFS) [J].

Brachmann, A ;

Geipel, G ;

Bernhard, G ;

Nitsche, H .

RADIOCHIMICA ACTA, 2002, 90 (03) :147-153

[5] A Family of UO22+-5-Nitro-1,3-dicarboxylate Hybrid Materials: Structural Variation As a Function of pH and Structure Directing Species [J].

Cantos, Paula M. ;

Cahill, Christopher L. .

CRYSTAL GROWTH & DESIGN, 2014, 14 (06) :3044-3053

[6] Three-Dimensional Polycatenation of a Uranium-Based Metal-Organic Cage: Structural Complexity and Radiation Detection [J].

Cheng, Liwei ;

Liang, Chengyu ;

Liu, Wei ;

Wang, Yaxing ;

Chen, Bin ;

Zhang, Hailong ;

Wang, Yanlong ;

Chai, Zhifang ;

Wang, Shuao .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2020, 142 (38) :16218-16222

[7] A series of uranium-organic frameworks: Crucial role of the protonation ability of auxiliary ligands [J].

Dai, Yong ;

Chai, Hui-Min ;

Zhang, Rui-Xin ;

Min, Jun-An ;

Wang, Zhao ;

Zhang, Meng ;

Zhang, Yu ;

Feng, Jing ;

Zhang, Chi ;

Wang, Juan .

INORGANIC CHEMISTRY COMMUNICATIONS, 2020, 111

[8] OLEX2: a complete structure solution, refinement and analysis program [J].

Dolomanov, Oleg V. ;

Bourhis, Luc J. ;

Gildea, Richard J. ;

Howard, Judith A. K. ;

Puschmann, Horst .

JOURNAL OF APPLIED CRYSTALLOGRAPHY, 2009, 42 :339-341

[9] A family of uranyl-aromatic dicarboxylate (pht-, ipa-, tpa-) framework hybrid materials: photoluminescence, surface photovoltage and dye adsorption [J].

Gao, Xue ;

Wang, Che ;

Shi, Zhong-Feng ;

Song, Jian ;

Bai, Feng-Ying ;

Wang, Ji-Xiao ;

Xing, Yong-Heng .

DALTON TRANSACTIONS, 2015, 44 (25) :11562-11571

[10] Dihydroxo-bridged diuranyl(vi) complexes with 2-((2-(6-chloropyridazin-3-yl)hydrazono)methyl)-4-R-phenols: structural insights and visible light driven photocatalytic activities [J].

Ghosh, Sabari ;

Srivastava, Ankit Kumar ;

Pal, Samudranil .

NEW JOURNAL OF CHEMISTRY, 2019, 43 (02) :970-978

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