Engineered Sorbents for Selective Uranium Sequestration from Seawater

被引:7
作者
Singh, Bhupendra Kumar [1 ,2 ]
Asim, Muhammad [1 ]
Salkenova, Zarina [1 ]
Pak, Donghun [1 ]
Um, Wooyong [1 ,2 ,3 ]
机构
[1] Pohang Univ Sci & Technol POSTECH, Div Adv Nucl Engn DANE, Pohang 790784, South Korea
[2] Pohang Univ Sci & Technol POSTECH, Nucl Environm Technol Inst NETI, Pohang 790784, South Korea
[3] Pohang Univ Sci & Technol POSTECH, Div Environm Sci & Engn DESE, Pohang 790784, South Korea
来源
ACS ES&T WATER | 2024年 / 4卷 / 02期
基金
新加坡国家研究基金会;
关键词
METAL-ORGANIC-FRAMEWORK; EXTRACTION; RECOVERY; ADSORPTION; SORPTION; NETWORK; U(VI); OXIDE; ARCHITECTURE; PROTEIN;
D O I
10.1021/acsestwater.3c00516
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The sustainable energy supply to the global community remains a great challenge due to the mounting incessant energy demand and environmental concerns associated with fossil fuel-based energy. As per the International Atomic Energy Agency (IAEA), nuclear power will be the only reliable sustainable energy source in the future, and there will be a high demand for uranium (U). Therefore, the exploitation of U from seawater is essential to supply nuclear energy for thousands of years globally. Herein, we discuss some key developments on the design and application of potential sorbents for effective uranium extraction from seawater (UES) under different experimental conditions. Specifically, we focus on the synthesis, characterization, and application of a) organic sorbents (metal-organic frameworks (MOFs), covalent organic frameworks (COFs), membranes, and hydrogels) and b) inorganic substrate (graphene and silica) based composite sorbents. Later, we discuss selected studies encompassing the mechanistic understating of efficient UES using potential sorbents through various analytical and theoretical/computational approaches. Finally, we present future challenges that need to be addressed for the design of compatible sorbents with exceptional properties for the effective UES. We believe that this paper can expand our understanding of the design and application of suitable sorbents for selective UES.
引用
收藏
页码:325 / 345
页数:21
相关论文
共 106 条
  • [1] Metal-Organic Framework Templated Inorganic Sorbents for Rapid and Efficient Extraction of Heavy Metals
    Abney, C. W.
    Gilhula, J. C.
    Lu, K.
    Lin, W.
    [J]. ADVANCED MATERIALS, 2014, 26 (47) : 7993 - +
  • [2] Materials for the Recovery of Uranium from Seawater
    Abney, Carter W.
    Mayes, Richard T.
    Saito, Tomonori
    Dai, Sheng
    [J]. CHEMICAL REVIEWS, 2017, 117 (23) : 13935 - 14013
  • [3] Polymer-Supported Bifunctional Amidoximes for the Sorption of Uranium from Seawater
    Alexandratos, Spiro D.
    Zhu, Xiaoping
    Florent, Marc
    Sellin, Remy
    [J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2016, 55 (15) : 4208 - 4216
  • [4] Novel Metal-Organic Framework (MOF) Based Composite Material for the Sequestration of U(VI) and Th(IV) Metal Ions from Aqueous Environment
    Alqadami, Ayoub Abdullah
    Naushad, Mu.
    Alothman, Zeid Abdullah
    Ghfar, Ayman A.
    [J]. ACS APPLIED MATERIALS & INTERFACES, 2017, 9 (41) : 36026 - 36037
  • [5] Diethylenetriamine tethered mesoporous silica for the sequestration of uranium from aqueous solution and seawater
    Amesh, P.
    Venkatesan, K. A.
    Suneesh, A. S.
    Samanta, Nibedita
    [J]. JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, 2020, 8 (04):
  • [6] Amidic succinic acid moiety anchored silica gel for the extraction of UO22+ from aqueous medium and simulated sea water
    Amesh, P.
    Suneesh, A. S.
    Selvan, B. Robert
    Venkatesan, K. A.
    [J]. COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS, 2019, 578
  • [7] Introduction of amino groups into acid-resistant MOFs for enhanced U(VI) sorption
    Bai, Zhi-Qiang
    Yuan, Li-Yong
    Zhu, Lin
    Liu, Zhi-Rong
    Chu, Sheng-Qi
    Zheng, Li-Rong
    Zhang, Jing
    Chai, Zhi-Fang
    Shi, Wei-Qun
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2015, 3 (02) : 525 - 534
  • [8] A novel 3D reticular anti-fouling bio-adsorbent for uranium extraction from seawater: Polyethylenimine and guanidyl functionalized hemp fibers
    Bai, Ziheng
    Liu, Qi
    Zhang, Hongsen
    Liu, Jingyuan
    Yu, Jing
    Wang, Jun
    [J]. CHEMICAL ENGINEERING JOURNAL, 2020, 382
  • [9] Removal of Trace Uranium from Groundwaters Using Membrane Capacitive Deionization Desalination for Potable Supply in Remote Communities: Bench, Pilot, and Field Scale Investigations
    Bales, Clare
    Kinsela, Andrew S. S.
    Miller, Christopher
    Wang, Yuan
    Zhu, Yunyi
    Lian, Boyue
    Waite, T. David
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2023, 57 (30) : 11345 - 11355
  • [10] Highly efficient antibacterial adsorbent for recovering uranium from seawater based on molecular structure design of PCN-222 post-engineering
    Bi, Changlong
    Zhang, Chunhong
    Xu, Wenda
    Ma, Fuqiu
    Zhu, Lien
    Zhu, Ruiqi
    Qi, Qi
    Liu, Lijia
    Bai, Jianwei
    Dong, Hongxing
    [J]. DESALINATION, 2023, 545