Facile synthesize of composite for pollutant removal of lead and methylene blue (MB)

被引:3
作者
Syed, Noureen [1 ,2 ,4 ]
Feng, Yongqiang [1 ]
Mahar, Faraz Khan [2 ]
Fahad, Raja [2 ]
Abro, Zamir Ahmed [3 ]
Huang, Jianfeng [1 ,4 ]
机构
[1] Shaanxi Univ Sci & Technol, Sch Mat Sci & Engn, Xian, Peoples R China
[2] Mehran Univ Engn & Technol, Dept Text Engn, Jamshoro, Pakistan
[3] Aror Univ, Art Architecture Design & Heritage, Sukker, Sindh, Pakistan
[4] Shaanxi Univ Sci & Technol, Sch Mat Sci & Engn, Xian 710021, Peoples R China
关键词
absorbency; lead removal; methylene blue; pectic enzymes; photocatalytic activity; CARBON QUANTUM DOTS; NANOMATERIALS; NITRIDE; WATER; PHOTOCATALYSTS; ENHANCEMENT; PERFORMANCE; DEGRADATION; CONVERSION; TIO2;
D O I
10.1002/ep.14317
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Water contamination caused by inconsistencies in the removal of contemporary colors and heavy metals constitutes a serious global ecological concern. This study introduces a composite material made of cellulose acetate coated with activated carbon, which is made more effective by including pectic enzymes. This composite is easily manufactured and has caused considerable interest due to its potential in wastewater treatment via absorption-based techniques for the photocatalytic degradation of methylene blue dye and lead removal. Thermal processing and electrospinning are used in the synthesis process. Field emission scanning electron microscopy (FE-SEM), Energy Dispersive Xray- Analysis (EDX), Brunauer-Emmett-Teller (BET), and UV-absorbency were used to characterize the resultant pectic cellulose/activated carbon nanofibers (P-CNFs). In addition, inductively coupled plasma-mass spectroscopy (ICP-MS) was used to evaluate lead ion adsorption. Several parameters, including initial lead ion and methylene blue concentrations, solution pH, and nanofiber, were investigated. Fifty percent of pectic-containing composite (cellulose/activated carbon) P-CNF has shown remarkable differences when compared to non-pectic and different ratio composite due to higher surface area and porosity. It also increases light absorption and decreases charge recombination, resulting in a maximum degradation efficiency of 98.5% in a neutral solution under UV-light irradiation for 25 min, compared to pure CNF (degradation efficiency is 49% after 60 min of irradiation). In the case of lead removal, 80% efficiency was achieved in 5 min.
引用
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页数:11
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  • [1] Insight into adsorption mechanism, modeling, and desirability function of crystal violet and methylene blue dyes by microalgae: Box-Behnken design application
    Abdulhameed, Ahmed Saud
    Jawad, Ali H.
    Kashi, Elmira
    Radzun, Khairul Adzfa
    ALOthman, Zeid A.
    Wilson, Lee D.
    [J]. ALGAL RESEARCH-BIOMASS BIOFUELS AND BIOPRODUCTS, 2022, 67
  • [2] Functionalized carbon-based nanomaterials and quantum dots with antibacterial activity: a review
    Alavi, Mehran
    Jabari, Erfan
    Jabbari, Esmaiel
    [J]. EXPERT REVIEW OF ANTI-INFECTIVE THERAPY, 2021, 19 (01) : 35 - 44
  • [3] Nickel ferrite-based composites and its photocatalytic application-A review
    Arumugham, Nagaveni
    Mariappan, Anusuya
    Eswaran, Jayanthi
    Daniel, Santhanaraj
    Kanthapazham, Rajakumar
    Kathirvel, Poonkodi
    [J]. JOURNAL OF HAZARDOUS MATERIALS ADVANCES, 2022, 8
  • [4] Enhanced oxidation ability of g-C3N4 photocatalyst via C60 modification
    Bai, Xiaojuan
    Wang, Li
    Wang, Yajun
    Yao, Wenqing
    Zhu, Yongfa
    [J]. APPLIED CATALYSIS B-ENVIRONMENTAL, 2014, 152 : 262 - 270
  • [5] Nanoagroparticles emerging trends and future prospect in modern agriculture system
    Baker, Syed
    Volova, Tatiana
    Prudnikova, Svetlana V.
    Satish, S.
    Prasad, Nagendra M. N.
    [J]. ENVIRONMENTAL TOXICOLOGY AND PHARMACOLOGY, 2017, 53 : 10 - 17
  • [6] Carbon-based H2-production photocatalytic materials
    Cao, Shaowen
    Yu, Jiaguo
    [J]. JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY C-PHOTOCHEMISTRY REVIEWS, 2016, 27 : 72 - 99
  • [7] Wavelength-dependent effects of carbon quantum dots on the photocatalytic activity of g-C3N4 enabled by LEDs
    Di, Guanglan
    Zhu, Zhiliang
    Dai, Qi
    Zhang, Hua
    Shen, Xiaolin
    Qiu, Yanling
    Huang, Yingying
    Yu, Jianan
    Yin, Daqiang
    Kueppers, Stephan
    [J]. CHEMICAL ENGINEERING JOURNAL, 2020, 379 (379)
  • [8] A critical review in strategies to improve photocatalytic water splitting towards hydrogen production
    Fajrina, Nur
    Tahir, Muhammad
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2019, 44 (02) : 540 - 577
  • [9] Z-scheme CdS/CQDs/g-C3N4 composites with visible-near-infrared light response for efficient photocatalytic organic pollutant degradation
    Feng, Shuting
    Chen, Tian
    Liu, Zhichao
    Shi, Jianhui
    Yue, Xiuping
    Li, Yuzhen
    [J]. SCIENCE OF THE TOTAL ENVIRONMENT, 2020, 704
  • [10] Green fabrication of citrus pectin-Ag@AgCl/g-C3N4 nanocomposites with enhanced photocatalytic activity for the degradation of new coccine
    Gong, Dezhuang
    Li, Xiquan
    Zhang, Xiuling
    Zhang, Wentao
    Chen, Tianhao
    Zhang, Xinhua
    [J]. FOOD CHEMISTRY, 2022, 387