Interfacial and surface magnetism in epitaxial NiCo2O4(001)/MgAl2O4 films

被引:8
作者
Mellinger, Corbyn [1 ]
Wang, Xiao [2 ]
Subedi, Arjun [1 ]
Clark, Andy T. [2 ]
Komesu, Takashi [1 ]
Rosenberg, Richard [3 ]
Dowben, Peter A. [1 ,4 ]
Cheng, Xuemei [2 ]
Xu, Xiaoshan [1 ,4 ]
机构
[1] Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA
[2] Bryn Mawr Coll, Dept Phys, Bryn Mawr, PA 19010 USA
[3] Argonne Natl Lab, Adv Photon Source, Lemont, IL 60439 USA
[4] Univ Nebraska, Nebraska Ctr Mat & Nanosci, Lincoln, NE 68588 USA
基金
美国国家科学基金会;
关键词
THIN-FILMS; INVERSE-PHOTOEMISSION; NICO2O4; ANISOTROPY; BEHAVIOR;
D O I
10.1063/5.0152539
中图分类号
O59 [应用物理学];
学科分类号
摘要
NiCo2O4 (NCO) films grown on MgAl2O4 (001) substrates have been studied using magnetometry and x-ray magnetic circular dichroism based on x-ray absorption spectroscopy and spin-polarized inverse photoemission spectroscopy with various thicknesses down to 1.6 nm. The magnetic behavior can be understood in terms of a layer of optimal NCO and an interfacial layer (1.2 +/- 0.1 nm), with a small canting of magnetization at the surface. The thickness dependence of the optimal layer can be described by the finite-scaling theory with a critical exponent consistent with the high perpendicular magnetic anisotropy. The interfacial layer couples antiferromagnetically to the optimal layer, generating exchange-spring styled magnetic hysteresis in the thinnest films. The non-optimal and measurement-speed-dependent magnetic properties of the interfacial layer suggest substantial interfacial diffusion.
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页数:7
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