zinc-air battery;
microbattery;
3D printing;
solid-state;
interdigital electrode;
gel polymer electrolyte;
HIGH-PERFORMANCE;
ENERGY;
ELECTRODES;
BATTERIES;
GRAPHENE;
ANODE;
D O I:
10.1021/acsami.2c22233
中图分类号:
TB3 [工程材料学];
学科分类号:
0805 ;
080502 ;
摘要:
Lightweight, compact, integrated, and miniaturized energy devices are under high pursuit for portable and wearable electronics. However, improving the energy density per area still remains a long-standing challenge. Herein, we report the design and fabrication of a solid-state zinc-air microbattery (ZAmB) by a facile 3D direct printing technique. The interdigital electrodes, gel electrolyte, and encapsulation frame are all printed with a customized design by optimzing the composition of the printing inks to obtain the best battery performance. Multiple layers of interdigital electrodes are sequentially printed with a fine overlap to achieve an ultrahigh thickness of 2.5 mm for a remarkably increased specific areal energy of up to 77.2 mWh cm-2. To meet the practical powering requirements for different output voltages and currents, battery modules consisting of individual ZAmBs connected in series or parallel or a combination of the two are printed with a facile integration to external loads. Powering of LEDs, digital watch, and a miniature rotary motor and even charging of a smartphone by the printed ZAmB modules are successfully demonstrated. The versatile 3D direct printing technique enables the fabricated ZAmBs with an adjustable form factor and integration capability with other electronics, paving the way for exploring new energy systems with diverse structures and extended functionalities.
机构:
Xi An Jiao Tong Univ, Xian 710049, Peoples R China
Qingdao Aerosp Power Struct Safety Inst, Qingdao 266580, Peoples R ChinaXi An Jiao Tong Univ, Xian 710049, Peoples R China
Wang, Yantao
Zhang, Xinyu
论文数: 0引用数: 0
h-index: 0
机构:
Qingdao Aerosp Power Struct Safety Inst, Qingdao 266580, Peoples R ChinaXi An Jiao Tong Univ, Xian 710049, Peoples R China
Zhang, Xinyu
Lang, Xianwei
论文数: 0引用数: 0
h-index: 0
机构:
Qingdao Aerosp Power Struct Safety Inst, Qingdao 266580, Peoples R ChinaXi An Jiao Tong Univ, Xian 710049, Peoples R China
Lang, Xianwei
Li, Zhi
论文数: 0引用数: 0
h-index: 0
机构:
Qingdao Aerosp Power Struct Safety Inst, Qingdao 266580, Peoples R ChinaXi An Jiao Tong Univ, Xian 710049, Peoples R China
Li, Zhi
Zhang, Chao
论文数: 0引用数: 0
h-index: 0
机构:
Qingdao Aerosp Power Struct Safety Inst, Qingdao 266580, Peoples R ChinaXi An Jiao Tong Univ, Xian 710049, Peoples R China
Zhang, Chao
Feng, Xingteng
论文数: 0引用数: 0
h-index: 0
机构:
Qingdao Aerosp Power Struct Safety Inst, Qingdao 266580, Peoples R ChinaXi An Jiao Tong Univ, Xian 710049, Peoples R China
Feng, Xingteng
Shi, Chuan
论文数: 0引用数: 0
h-index: 0
机构:
Qingdao Univ, Coll Phys, Qingdao 266071, Peoples R ChinaXi An Jiao Tong Univ, Xian 710049, Peoples R China
机构:
Ningxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R ChinaNingxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R China
Liu, Xiaoyi
Wang, Jian
论文数: 0引用数: 0
h-index: 0
机构:
Ningxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R ChinaNingxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R China
Wang, Jian
Wu, Bintao
论文数: 0引用数: 0
h-index: 0
机构:
Ningxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R ChinaNingxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R China
Wu, Bintao
Li, Haibo
论文数: 0引用数: 0
h-index: 0
机构:
Ningxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R ChinaNingxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R China
Li, Haibo
Ma, Pin
论文数: 0引用数: 0
h-index: 0
机构:
Ningxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R ChinaNingxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R China
Ma, Pin
Yang, Hui Ying
论文数: 0引用数: 0
h-index: 0
机构:
Singapore Univ Technol & Design, Pillar Engn Prod Dev, 8 Somapah Rd, Singapore 487372, SingaporeNingxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R China
机构:
Xi An Jiao Tong Univ, Xian 710049, Peoples R China
Qingdao Aerosp Power Struct Safety Inst, Qingdao 266580, Peoples R ChinaXi An Jiao Tong Univ, Xian 710049, Peoples R China
Wang, Yantao
Zhang, Xinyu
论文数: 0引用数: 0
h-index: 0
机构:
Qingdao Aerosp Power Struct Safety Inst, Qingdao 266580, Peoples R ChinaXi An Jiao Tong Univ, Xian 710049, Peoples R China
Zhang, Xinyu
Lang, Xianwei
论文数: 0引用数: 0
h-index: 0
机构:
Qingdao Aerosp Power Struct Safety Inst, Qingdao 266580, Peoples R ChinaXi An Jiao Tong Univ, Xian 710049, Peoples R China
Lang, Xianwei
Li, Zhi
论文数: 0引用数: 0
h-index: 0
机构:
Qingdao Aerosp Power Struct Safety Inst, Qingdao 266580, Peoples R ChinaXi An Jiao Tong Univ, Xian 710049, Peoples R China
Li, Zhi
Zhang, Chao
论文数: 0引用数: 0
h-index: 0
机构:
Qingdao Aerosp Power Struct Safety Inst, Qingdao 266580, Peoples R ChinaXi An Jiao Tong Univ, Xian 710049, Peoples R China
Zhang, Chao
Feng, Xingteng
论文数: 0引用数: 0
h-index: 0
机构:
Qingdao Aerosp Power Struct Safety Inst, Qingdao 266580, Peoples R ChinaXi An Jiao Tong Univ, Xian 710049, Peoples R China
Feng, Xingteng
Shi, Chuan
论文数: 0引用数: 0
h-index: 0
机构:
Qingdao Univ, Coll Phys, Qingdao 266071, Peoples R ChinaXi An Jiao Tong Univ, Xian 710049, Peoples R China
机构:
Ningxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R ChinaNingxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R China
Liu, Xiaoyi
Wang, Jian
论文数: 0引用数: 0
h-index: 0
机构:
Ningxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R ChinaNingxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R China
Wang, Jian
Wu, Bintao
论文数: 0引用数: 0
h-index: 0
机构:
Ningxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R ChinaNingxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R China
Wu, Bintao
Li, Haibo
论文数: 0引用数: 0
h-index: 0
机构:
Ningxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R ChinaNingxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R China
Li, Haibo
Ma, Pin
论文数: 0引用数: 0
h-index: 0
机构:
Ningxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R ChinaNingxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R China
Ma, Pin
Yang, Hui Ying
论文数: 0引用数: 0
h-index: 0
机构:
Singapore Univ Technol & Design, Pillar Engn Prod Dev, 8 Somapah Rd, Singapore 487372, SingaporeNingxia Univ, Sch Mat & New Energy, Ningxia Key Lab Photovolta Mat, Yinchuan 750021, Peoples R China