This study investigated the production of hydrogen-rich syngas from renewable sources using durable and efficient catalysts. Specifically, the research focused on steam methane reforming (SRM) and dry methane reforming (DRM) of simulated producer gas from biomass steam gasification in a fluidized bed reactor. The catalysts tested are ZSM-5-supported nickel-iron-cobalt-based trimetallic catalysts in different ratios, which were prepared via the wet impregnation method. Synthesized catalysts were characterized using XRD, BET, H2-TPR, and SEM techniques. The results of the SRM with the simulated producer gas showed that the 20%Ni-20%Fe-10%Co/ZSM-5 trimetallic catalyst, at a gas hourly space velocity (GHSV) of 12 L center dot h-1 center dot g-1 and reaction temperature of 800 degrees C, achieved the highest CH4 conversion (74.8%) and highest H2 yield (65.59%) with CO2 conversion (36.05%). Comparing the performance of the SRM and DRM of the simulated producer gas with the 20%Ni-20%Fe-10%Co/ZSM5 at a GHSV of 36 L center dot h-1 center dot g-1 and 800 degrees C, they achieved a CH4 conversion of 67.18% and 64.43%, a CO2 conversion of 43.01% and 52.1%, and a H2 yield of 55.49% and 42.02%, respectively. This trimetallic catalyst demonstrated effective inhibition of carbon formation and sintering, with only 2.6 wt.% carbon deposition observed from the thermo-gravimetric analysis of the used catalyst from the SRM of the simulated producer gas, thus promoting the potential of the ZSM-5-supported trimetallic catalysts in methane reforming.
机构:
Univ Putra Malaysia, Fac Sci, Catalysis Sci & Technol Res Ctr, Serdang 43400, Selangor, Malaysia
Univ Putra Malaysia, Fac Sci, Dept Chem, Serdang 43400, Selangor, MalaysiaUniv Putra Malaysia, Fac Sci, Catalysis Sci & Technol Res Ctr, Serdang 43400, Selangor, Malaysia
Al-Doghachi, Faris A. J.
;
Rashid, Umer
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Univ Putra Malaysia, Inst Adv Technol, Serdang 43400, Selangor, MalaysiaUniv Putra Malaysia, Fac Sci, Catalysis Sci & Technol Res Ctr, Serdang 43400, Selangor, Malaysia
Rashid, Umer
;
Taufiq-Yap, Yun Hin
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Univ Putra Malaysia, Fac Sci, Catalysis Sci & Technol Res Ctr, Serdang 43400, Selangor, Malaysia
Univ Putra Malaysia, Fac Sci, Dept Chem, Serdang 43400, Selangor, MalaysiaUniv Putra Malaysia, Fac Sci, Catalysis Sci & Technol Res Ctr, Serdang 43400, Selangor, Malaysia
机构:
Univ Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, IranUniv Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
Bayat, Nima
;
Rezaei, Mehran
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Univ Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
Univ Kashan, Inst Nanosci & Nanotechnol, Kashan, IranUniv Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
Rezaei, Mehran
;
Meshkani, Fereshteh
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Univ Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, IranUniv Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
机构:
Univ Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, IranUniv Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
Bayat, Nima
;
Rezaei, Mehran
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Univ Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
Univ Kashan, Inst Nanosci & Nanotechnol, Kashan, IranUniv Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
Rezaei, Mehran
;
Meshkani, Fereshteh
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Univ Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, IranUniv Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
机构:
Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA
Chen, Luning
;
Qi, Zhiyuan
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机构:
Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA
Qi, Zhiyuan
;
Zhang, Shuchen
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机构:
Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA
Zhang, Shuchen
;
Su, Ji
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机构:
Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA
Lawrence Berkeley Natl Lab, Mat Sci Div, Mol Foundry, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA
Su, Ji
;
Somorjai, Gabor A.
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机构:
Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA
机构:
Univ Putra Malaysia, Fac Sci, Catalysis Sci & Technol Res Ctr, Serdang 43400, Selangor, Malaysia
Univ Putra Malaysia, Fac Sci, Dept Chem, Serdang 43400, Selangor, MalaysiaUniv Putra Malaysia, Fac Sci, Catalysis Sci & Technol Res Ctr, Serdang 43400, Selangor, Malaysia
Al-Doghachi, Faris A. J.
;
Rashid, Umer
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h-index: 0
机构:
Univ Putra Malaysia, Inst Adv Technol, Serdang 43400, Selangor, MalaysiaUniv Putra Malaysia, Fac Sci, Catalysis Sci & Technol Res Ctr, Serdang 43400, Selangor, Malaysia
Rashid, Umer
;
Taufiq-Yap, Yun Hin
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h-index: 0
机构:
Univ Putra Malaysia, Fac Sci, Catalysis Sci & Technol Res Ctr, Serdang 43400, Selangor, Malaysia
Univ Putra Malaysia, Fac Sci, Dept Chem, Serdang 43400, Selangor, MalaysiaUniv Putra Malaysia, Fac Sci, Catalysis Sci & Technol Res Ctr, Serdang 43400, Selangor, Malaysia
机构:
Univ Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, IranUniv Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
Bayat, Nima
;
Rezaei, Mehran
论文数: 0引用数: 0
h-index: 0
机构:
Univ Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
Univ Kashan, Inst Nanosci & Nanotechnol, Kashan, IranUniv Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
Rezaei, Mehran
;
Meshkani, Fereshteh
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h-index: 0
机构:
Univ Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, IranUniv Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
机构:
Univ Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, IranUniv Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
Bayat, Nima
;
Rezaei, Mehran
论文数: 0引用数: 0
h-index: 0
机构:
Univ Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
Univ Kashan, Inst Nanosci & Nanotechnol, Kashan, IranUniv Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
Rezaei, Mehran
;
Meshkani, Fereshteh
论文数: 0引用数: 0
h-index: 0
机构:
Univ Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, IranUniv Kashan, Dept Chem Engn, Catalyst & Adv Mat Res Lab, Fac Engn, Kashan, Iran
机构:
Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA
Chen, Luning
;
Qi, Zhiyuan
论文数: 0引用数: 0
h-index: 0
机构:
Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA
Qi, Zhiyuan
;
Zhang, Shuchen
论文数: 0引用数: 0
h-index: 0
机构:
Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA
Zhang, Shuchen
;
Su, Ji
论文数: 0引用数: 0
h-index: 0
机构:
Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA
Lawrence Berkeley Natl Lab, Mat Sci Div, Mol Foundry, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA
Su, Ji
;
Somorjai, Gabor A.
论文数: 0引用数: 0
h-index: 0
机构:
Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USALawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA