Upgrading the detection of electrocatalyst degradation during the oxygen evolution reaction

被引:17
作者
Risch, Marcel [1 ]
机构
[1] Helmholtz Zent Berlin Mat & Energie GmbH, Nachwuchsgrp Gestaltung Sauer Stoffentwicklungsmec, Hahn Meitner Pl 1, D-14019 Berlin, Germany
基金
欧洲研究理事会;
关键词
Electrocatalysis; Oxygen evolution reaction; Corrosion; Electrocatalyst degradation; Mechanisms; Best practices; RATIONAL DESIGN; STABILITY; BENCHMARKING; OXIDATION; DISSOLUTION; MICROSCOPY; CATALYSTS; OXIDES;
D O I
10.1016/j.coelec.2023.101247
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Electrocatalysts for the oxygen evolution reaction (OER) are an important component for the transition from fossil to sus-tainable energy. Commercialization of cost-effective earth -abundant electrocatalysts is in large parts hindered by their degradation. In this short review, I identify common processes leading to a decrease in electrocatalyst activity, followed by an introduction of staple methods to determine degradation electrochemically and by additional physical characterization, which has the potential to remove ambiguities of purely elec-trochemical studies. I conclude by a summary of the key challenges for an accurate determination of degradation pro-cesses and highlight interesting directions to advance the un-derstanding of degradation processes on electrocatalysts in materials-centered model studies.
引用
收藏
页数:10
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