Stabilizing CsPbI3 perovskite for photovoltaic applications

被引：51
作者：
Tan, Xue [1 ]
Wang, Shubin [1 ]
Zhang, Qixian [1 ]
Liu, Huicong [1 ]
Li, Weiping [1 ]
Zhu, Liqun [1 ]
Chen, Haining [1 ]
机构：
[1] Beihang Univ, Sch Mat Sci & Engn, 37 Xueyuan Rd, Beijing 100191, Peoples R China
来源：
MATTER | 2023年 / 6卷 / 03期
基金：
中国国家自然科学基金; 北京市自然科学基金;
关键词：
CESIUM LEAD IODIDE; HALIDE PEROVSKITES; SOLAR-CELLS; ALPHA-CSPBI3; PEROVSKITE; ELECTRONIC-PROPERTIES; PHASE-TRANSITION; EFFICIENT; NANOCRYSTALS; PERFORMANCE; BR;
D O I：
10.1016/j.matt.2022.12.012
中图分类号：
T [工业技术];
学科分类号：
08 ;
摘要：
With suitable band gap (Eg -1.7 eV), superb optoelectronic proper-ties, and thermal stability, CsPbI3 has been widely acknowledged as a competitive candidate for photovoltaic devices. However, the spontaneous phase transition to a non-perovskite phase limits its further application. Mighty efforts and advances have been made to stabilize the perovskite structure of CsPbI3 and improve power conversion efficiency of perovskite solar cells. In this review, we give insights regarding the origin of the instability of CsPbI3 from intrinsic assessment to external stimulation and review the strate-gies and progress to improve the stability of CsPbI3 perovskite structure and devices from the following aspects: (1) ionic incorpo-ration, (2) regulating surface energy, (3) incorporating low-dimen-sional perovskites, and (4) surface termination. Finally, we give a brief outlook on the challenges and opportunities of all-inorganic CsPbI3 perovskite.
引用
收藏
页码：691 / 727
页数：37
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