Process intensification;
Intensification of mass and heat transfer;
Stationary bed reactor;
Rotating bed reactor;
Heterogeneous biocatalysts;
A novel design of reactor;
ESTER SYNTHESIS;
MASS-TRANSFER;
CATALYST;
D O I:
10.1016/j.cep.2023.109590
中图分类号:
TE [石油、天然气工业];
TK [能源与动力工程];
学科分类号:
0807 ;
0820 ;
摘要:
Effectiveness of catalytic processes using heterogeneous biocatalysts depends not only on the activity of the enzyme, but also on the efficiency of the used reactor. In this paper, we present a novel design of a basket reactor with a stationary catalyst bed (StatBioChem). The developed design was compared to a commercially available rotating bed reactor (SpinChem (R)). The biocatalysts used were invertase and acyltransferase from Mycobacterium smegmatis (MsAcT) immobilised on macroporous silica supports. The obtained values of initial reaction rate, both in the reaction of saccharose hydrolysis and 2,2-dimethyl-1,3-propanediol (NPG) transesterification, were twice higher for the StatBioChem reactor. A similar relationship was also observed regarding the process efficiency expressed as STY.
机构:
CNRS, UMR 7285, Inst Chim Milieux & Mat Poitiers, 4 Rue Michel Brunet,Batiment B27, F-86073 Poitiers 9, FranceCNRS, UMR 7285, Inst Chim Milieux & Mat Poitiers, 4 Rue Michel Brunet,Batiment B27, F-86073 Poitiers 9, France
Astafan, Amir
Sachse, Alexander
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机构:
CNRS, UMR 7285, Inst Chim Milieux & Mat Poitiers, 4 Rue Michel Brunet,Batiment B27, F-86073 Poitiers 9, FranceCNRS, UMR 7285, Inst Chim Milieux & Mat Poitiers, 4 Rue Michel Brunet,Batiment B27, F-86073 Poitiers 9, France
Sachse, Alexander
Batiot-Dupeyrat, Catherine
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机构:
CNRS, UMR 7285, Inst Chim Milieux & Mat Poitiers, 4 Rue Michel Brunet,Batiment B27, F-86073 Poitiers 9, FranceCNRS, UMR 7285, Inst Chim Milieux & Mat Poitiers, 4 Rue Michel Brunet,Batiment B27, F-86073 Poitiers 9, France
Batiot-Dupeyrat, Catherine
Pinard, Ludovic
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机构:
CNRS, UMR 7285, Inst Chim Milieux & Mat Poitiers, 4 Rue Michel Brunet,Batiment B27, F-86073 Poitiers 9, FranceCNRS, UMR 7285, Inst Chim Milieux & Mat Poitiers, 4 Rue Michel Brunet,Batiment B27, F-86073 Poitiers 9, France
机构:
Hokkaido Univ, Fac Engn, Div Chem Proc Engn, Kita Ku, Sapporo, Hokkaido 0608628, JapanHokkaido Univ, Fac Engn, Div Chem Proc Engn, Kita Ku, Sapporo, Hokkaido 0608628, Japan
Nakasaka, Yuta
Tago, Teruoki
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机构:
Hokkaido Univ, Fac Engn, Div Chem Proc Engn, Kita Ku, Sapporo, Hokkaido 0608628, JapanHokkaido Univ, Fac Engn, Div Chem Proc Engn, Kita Ku, Sapporo, Hokkaido 0608628, Japan
Tago, Teruoki
Konno, Hiroki
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Hokkaido Univ, Fac Engn, Div Chem Proc Engn, Kita Ku, Sapporo, Hokkaido 0608628, JapanHokkaido Univ, Fac Engn, Div Chem Proc Engn, Kita Ku, Sapporo, Hokkaido 0608628, Japan
Konno, Hiroki
Okabe, Akihiro
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机构:
Mitsui Chem Inc, Catalysis Sci Lab, Sodegaura, Chiba 2990265, JapanHokkaido Univ, Fac Engn, Div Chem Proc Engn, Kita Ku, Sapporo, Hokkaido 0608628, Japan
Okabe, Akihiro
Masuda, Takao
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机构:
Hokkaido Univ, Fac Engn, Div Chem Proc Engn, Kita Ku, Sapporo, Hokkaido 0608628, JapanHokkaido Univ, Fac Engn, Div Chem Proc Engn, Kita Ku, Sapporo, Hokkaido 0608628, Japan