Enhancement of spontaneous emission from CdSe/ZnS quantum dots through silicon nitride photonic crystal cavity based on miniaturized bound states in the continuum

被引:5
作者
Qiu, Guixin [1 ]
Wei, Dunzhao [1 ]
Liu, Zhuojun [2 ]
Liu, Jin [1 ]
机构
[1] Sun Yat Sen Univ, Sch Phys, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Peoples R China
[2] Peking Univ, Ctr Nanooptoelectron, Sch Phys, State Key Lab Mesoscop Phys & Frontiers Sci, Beijing 100871, Peoples R China
基金
中国博士后科学基金; 中国国家自然科学基金;
关键词
LIGHT-EMITTING-DIODES; 2ND-HARMONIC GENERATION; FLUORESCENCE; EFFICIENCY; LASERS; ROBUST;
D O I
10.1039/d2nr05031e
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Colloidal CdSe/ZnS quantum dots (QDs) exhibit excellent optical properties for wide potential applications in light-emitting diodes, solar concentrators, and single-photon sources. However, the ultra-thin films with low concentration of QDs still encounter inefficient photoluminescence (PL) and poor directionality of radiation, which need to be enhanced using nanophotonics device designs. Here we design and experimentally demonstrate an on-substrate silicon nitride (SiN) photonic crystal (PhC) microcavity encapsulated by a layer of PMMA hosting CdSe/ZnS QDs. The miniaturized bound states in the continuum (BIC) supported by our structures, provide high-Q resonant modes with highly-directional emission patterns. Experimental results show that the BIC mode in the microcavity has a Q-factor up to 7000 owing to the symmetric refractive index distribution along the Z-direction, rendering 8.5-fold enhancement of PL intensity and 8.4-fold acceleration of radiative emission rate. Our work provides a practical way for constructing efficient on-chip surface-emitting light sources on silicon-based integrated photonic devices.
引用
收藏
页码:3757 / 3763
页数:8
相关论文
共 43 条
  • [11] CMOS Compatible High-Performance Nanolasing Based on Perovskite-SiN Hybrid Integration
    He, Zhe
    Chen, Bo
    Hua, Yan
    Liu, Zhuojun
    Wei, Yuming
    Liu, Shunfa
    Hu, An
    Shen, Xinyu
    Zhang, Yu
    Gao, Yunan
    Liu, Jin
    [J]. ADVANCED OPTICAL MATERIALS, 2020, 8 (15)
  • [12] Synthesis and characterization of strongly luminescing ZnS-Capped CdSe nanocrystals
    Hines, MA
    Guyot-Sionnest, P
    [J]. JOURNAL OF PHYSICAL CHEMISTRY, 1996, 100 (02) : 468 - 471
  • [13] Bound states in the continuum
    Hsu, Chia Wei
    Zhen, Bo
    Stone, A. Douglas
    Joannopoulos, John D.
    Soljacic, Marin
    [J]. NATURE REVIEWS MATERIALS, 2016, 1 (09):
  • [14] Ultrafast control of vortex microlasers
    Huang, Can
    Zhang, Chen
    Xiao, Shumin
    Wang, Yuhan
    Fan, Yubin
    Liu, Yilin
    Zhang, Nan
    Qu, Geyang
    Ji, Hongjun
    Han, Jiecai
    Ge, Li
    Kivshar, Yuri
    Song, Qinghai
    [J]. SCIENCE, 2020, 367 (6481) : 1018 - +
  • [15] Ultralow-threshold laser using super-bound states in the continuum
    Hwang, Min-Soo
    Lee, Hoo-Cheol
    Kim, Kyoung-Ho
    Jeong, Kwang-Yong
    Kwon, Soon-Hong
    Koshelev, Kirill
    Kivshar, Yuri
    Park, Hong-Gyu
    [J]. NATURE COMMUNICATIONS, 2021, 12 (01)
  • [16] Topologically enabled ultrahigh-Q guided resonances robust to out-of-plane scattering
    Jin, Jicheng
    Yin, Xuefan
    Ni, Liangfu
    Soljacic, Marin
    Zhen, Bo
    Peng, Chao
    [J]. NATURE, 2019, 574 (7779) : 501 - +
  • [17] Colloidal quantum dots in all-dielectric high-Q pillar microcavities
    Kahl, Matthias
    Thomay, Tim
    Kohnle, Verena
    Beha, Katja
    Merlein, Jorg
    Hagner, Matthias
    Halm, Andreas
    Ziegler, Jan
    Nann, Thomas
    Fedutik, Yuri
    Woggon, Ulrike
    Artemyev, Mikhail
    Perez-Willard, Fabian
    Leitenstorfer, Alfred
    Bratschitsch, Rudolf
    [J]. NANO LETTERS, 2007, 7 (09) : 2897 - 2900
  • [18] Meta-optics and bound states in the continuum
    Koshelev, Kirill
    Bogdanov, Andrey
    Kivshar, Yuri
    [J]. SCIENCE BULLETIN, 2019, 64 (12) : 836 - 842
  • [19] Asymmetric parametric generation of images with nonlinear dielectric metasurfaces
    Kruk, Sergey S.
    Wang, Lei
    Sain, Basudeb
    Dong, Zhaogang
    Yang, Joel
    Zentgraf, Thomas
    Kivshar, Yuri
    [J]. NATURE PHOTONICS, 2022, 16 (08) : 561 - +
  • [20] Enhanced luminescence of CdSe quantum dots on gold colloids
    Kulakovich, O
    Strekal, N
    Yaroshevich, A
    Maskevich, S
    Gaponenko, S
    Nabiev, I
    Woggon, U
    Artemyev, M
    [J]. NANO LETTERS, 2002, 2 (12) : 1449 - 1452