Enhanced mechanical and electrical properties of starch-based hydrogels incorporating polyacrylic acid and MXene for advanced wearable sensors in sign language recognition

被引:6
作者
Liang, Jionghong [1 ,2 ]
Ma, Ke [1 ]
Gao, Wenshuo [1 ]
Xin, Yue [1 ]
Chen, Shousen [1 ]
Qiu, Weicheng [1 ]
Shen, Gengzhe [3 ]
He, Xin [1 ]
机构
[1] Wuyi Univ, Sch Appl Phys & Mat, Jiangmen 529020, Peoples R China
[2] Guangdong Univ Technol, Sch Electromech Engn, Guangzhou 510006, Peoples R China
[3] Chinese Acad Sci, Zhuhai Inst Adv Technol, Zhuhai 519003, Peoples R China
来源
SENSORS & DIAGNOSTICS | 2024年 / 3卷 / 02期
关键词
STRAIN; DESIGN; ADHESIVE; TOUGH; SKIN;
D O I
10.1039/d3sd00250k
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
Traditional starch-based hydrogels often lack the mechanical robustness and electrical conductivity required for strain sensing applications. In this study, a conductive organohydrogel was developed by blending starch and MXene with polyacrylic acid (PAA). The resulting PAA/starch/MXene organohydrogel exhibits exceptional mechanical strength, high electrical conductivity, robust adhesion, and resilience to low temperatures. Strain sensors based on this innovative material demonstrate remarkable characteristics, including high sensitivity (maximum GF = 14.19), rapid response time (approximately 160 ms), a wide sensing range (exceeding 800%), and excellent cycling stability. Notably, these sensors remain efficient even at frigid temperatures as low as -30 degrees C. Furthermore, these sensors find practical application in sign language translation, achieving an impressive recognition rate of up to 100% for complex sentences. When integrated into a sensor array, they enable precise assessment of load magnitude and distribution. Consequently, this research introduces an innovative strategy for fabricating highly efficient conductive hydrogels, holding significant promise for diverse applications in the realm of flexible electronic devices, and promoting sustainable advancements in the field of wearable electronics. A PAA/Starch/MXene organohydrogel was developed for strain sensors with remarkable sensitivity, offering potential for widespread applications in wearable electronics.
引用
收藏
页码:256 / 268
页数:13
相关论文
共 57 条
[1]   Design and development of trivalent aluminum ions induced self healing polyacrylic acid novel hydrogels [J].
Anjum, Sadiya ;
Gurave, Pramod ;
Badiger, Manohar V. ;
Torris, Arun ;
Tiwari, Neha ;
Gupta, Bhuvanesh .
POLYMER, 2017, 126 :196-205
[2]   RETROGRADATION KINETICS OF WAXY-CORN AND POTATO STARCHES - A RAPID, RAMAN-SPECTROSCOPIC STUDY [J].
BULKIN, BJ ;
KWAK, Y ;
DEA, ICM .
CARBOHYDRATE RESEARCH, 1987, 160 :95-112
[3]   Multiple-Stimuli-Responsive and Cellulose Conductive Ionic Hydrogel for Smart Wearable Devices and Thermal Actuators [J].
Chen, Zhen ;
Liu, Jing ;
Chen, Yujie ;
Zheng, Xu ;
Liu, Hezhou ;
Li, Hua .
ACS APPLIED MATERIALS & INTERFACES, 2021, 13 (01) :1353-1366
[4]  
Chortos A, 2016, NAT MATER, V15, P937, DOI [10.1038/nmat4671, 10.1038/NMAT4671]
[5]   All-Lignin-Based Hydrogel with Fast pH-Stimuli Responsiveness for Mechanical Switching and Actuation [J].
Dai, Lin ;
Ma, Mingshuai ;
Xu, Jikun ;
Si, Chuanling ;
Wang, Xiaohui ;
Liu, Zhong ;
Ni, Yonghao .
CHEMISTRY OF MATERIALS, 2020, 32 (10) :4324-4330
[6]   Poly(N-isopropylacrylamide)-SiO2 nanocomposites interpenetrated by starch: Stimuli-responsive hydrogels with attractive tensile properties [J].
Depa, Katarzyna ;
Strachota, Adam ;
Slouf, Miroslav ;
Brus, Jiri .
EUROPEAN POLYMER JOURNAL, 2017, 88 :349-372
[7]   Mussel foot protein inspired tough tissue-selective underwater adhesive hydrogel [J].
Fan, Xianmou ;
Fang, Yan ;
Zhou, Weikang ;
Yan, Liyu ;
Xu, Yuehua ;
Zhu, Hu ;
Liu, Haiqing .
MATERIALS HORIZONS, 2021, 8 (03) :997-1007
[8]   A hydrogel sensor driven by sodium carboxymethyl starch with synergistic enhancement of toughness and conductivity [J].
Gao, Yiyan ;
Zhang, Zhixin ;
Ren, Xiuyan ;
Jia, Fei ;
Gao, Guanghui .
JOURNAL OF MATERIALS CHEMISTRY B, 2022, 10 (30) :5743-5752
[9]   Mechanical, adhesive and self-healing ionic liquid hydrogels for electrolytes and flexible strain sensors [J].
Gao, Zijian ;
Kong, Lingshu ;
Jin, Rining ;
Liu, Xin ;
Hu, Wei ;
Gao, Guanghui .
JOURNAL OF MATERIALS CHEMISTRY C, 2020, 8 (32) :11119-11127
[10]   Ti3C2Tx MXene-Activated Fast Gelation of Stretchable and Self-Healing Hydrogels: A Molecular Approach [J].
Ge, Gang ;
Zhang, Yi-Zhou ;
Zhang, Wenli ;
Yuan, Wei ;
El-Demellawi, Jehad K. ;
Zhang, Peng ;
Di Fabrizio, Enzo ;
Dong, Xiaochen ;
Alshareef, Husam N. .
ACS NANO, 2021, 15 (02) :2698-2706