Influencing factors identification and the nested structure analysis of heavy metals in soils in entire city and surrounding the multiple pollution sources

被引:21
作者
Qiao, Pengwei [1 ]
Wang, Shuo [1 ]
Lei, Mei [2 ]
Guo, Guanghui [2 ]
Yang, Jun [2 ]
Wei, Yan [1 ]
Gou, Yaling [1 ]
Li, Peizhong [1 ]
Zhang, Zhongguo [1 ]
机构
[1] Beijing Acad Sci & Technol, Inst Resources & Environm, Beijing Key Lab Remediat Ind Pollut Sites, Beijing 100089, Peoples R China
[2] Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Beijing 100101, Peoples R China
关键词
Soil pollution; Quantitative analysis; Nested semivariogram; Random forest; Positive matrix factorization; POSITIVE MATRIX FACTORIZATION; HEALTH-RISK ASSESSMENT; SOURCE APPORTIONMENT; URBAN SOILS; ROAD DUST; AREA; ACCUMULATION; REGRESSION; EMISSIONS; PATTERN;
D O I
10.1016/j.jhazmat.2023.130961
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Identifying the sources of pollutants and analyzing the nested structure of heavy metals is vital for the prevention and control of soil pollution. However, there is a lack of research on comparison the main sources and the nested structure at different scales. In this study, two spatial extent scales were taken as the research objects, the results showed that, (1) the point exceeding standard rate of As, Cr, Ni, and Pb is higher at the entire city scale; (2) As and Pb, while Cr, Ni, and Zn, have weaker spatial variability at the entire scale and surrounding the pollution sources, respectively; (3) the contribution of the larger structure of Cr and Ni, while Cr, Ni, and Zn, at the entire scale and surrounding the pollution sources, respectively, is bigger to the total variability. The representation of semivariogram is better when the general spatial variability is weaker and the contribution of the smaller structure is lower; (4) various factors with different influencing distance could lead to nested structure even at a small extent spatial scale. The results provide a basis for the determination of remediation and prevention ob-jectives at different spatial scales.
引用
收藏
页数:14
相关论文
共 46 条
[1]   Contamination characteristics and source apportionment of heavy metals in topsoil from an area in Xi'an city, China [J].
Chen, Xiuduan ;
Lu, Xinwei .
ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY, 2018, 151 :153-+
[2]   Scale-dependent spatial heterogeneity of vegetation in Mu Us sandy land, a semi-arid area of China [J].
Chen, YF ;
Yu, FH ;
Dong, M .
PLANT ECOLOGY, 2002, 162 (01) :135-142
[3]   Comparisons of two serious air pollution episodes in winter and summer in Beijing [J].
Cheng, Nianliang ;
Li, Yunting ;
Cheng, Bingfen ;
Wang, Xin ;
Meng, Fan ;
Wang, Qin ;
Qiu, Qihong .
JOURNAL OF ENVIRONMENTAL SCIENCES, 2018, 69 :141-154
[4]   Assessment of air pollution caused by illegal e-waste burning to evaluate the human health risk [J].
Gangwar, Charu ;
Choudhari, Ranjana ;
Chauhan, Anju ;
Kumar, Atul ;
Singh, Aprajita ;
Tripathi, Anamika .
ENVIRONMENT INTERNATIONAL, 2019, 125 :191-199
[5]   The interpolation accuracy for seven soil properties at various sampling scales on the Loess Plateau, China [J].
Gao, Lei ;
Shao, Mingan .
JOURNAL OF SOILS AND SEDIMENTS, 2012, 12 (02) :128-142
[6]   The power of Random Forest for the identification and quantification of technogenic substrates in urban soils on the basis of DRIFT spectra [J].
Heil, Jannis ;
Michaelis, Xandra ;
Marschner, Bernd ;
Stumpe, Britta .
ENVIRONMENTAL POLLUTION, 2017, 230 :574-583
[7]   Quantitative source apportionment of heavy metal(loid)s in the agricultural soils of an industrializing region and associated model uncertainty [J].
Hu, Yuanan ;
He, Kailing ;
Sun, Zehang ;
Chen, Gang ;
Cheng, Hefa .
JOURNAL OF HAZARDOUS MATERIALS, 2020, 391
[8]   Identification of the potential risk areas for soil heavy metal pollution based on the source-sink theory [J].
Jia, Xiaolin ;
Fu, Tingting ;
Hu, Bifeng ;
Shi, Zhou ;
Zhou, Lianqing ;
Zhu, Youwei .
JOURNAL OF HAZARDOUS MATERIALS, 2020, 393
[9]   VIRS based detection in combination with machine learning for mapping soil pollution [J].
Jia, Xiyue ;
O'Connor, David ;
Shi, Zhou ;
Hou, Deyi .
ENVIRONMENTAL POLLUTION, 2021, 268
[10]   Source apportionment and health risk assessment of heavy metals in soil for a township in Jiangsu Province, China [J].
Jiang, Yanxue ;
Chao, Sihong ;
Liu, Jianwei ;
Yang, Yue ;
Chen, Yanjiao ;
Zhang, Aichen ;
Cao, Hongbin .
CHEMOSPHERE, 2017, 168 :1658-1668