Gradient Bandgap-Tunable Perovskite Microwire Arrays toward Flexible Color-Cognitive Devices

被引:53
作者
Fu, Yue [1 ]
Yuan, Meng [2 ,3 ]
Zhao, Yingjie [4 ]
Dong, Meiqiu [1 ]
Guo, Yangwu [1 ]
Wang, Kui [1 ]
Jin, Chunqi [5 ]
Feng, Jiangang [6 ]
Wu, Yuchen [1 ,2 ]
Jiang, Lei [2 ]
机构
[1] Ji Hua Lab, Foshan 528200, Guangdong, Peoples R China
[2] Chinese Acad Sci, Tech Inst Phys & Chem, Key Lab Bioinspired Mat & Interfacial Sci, Beijing 100190, Peoples R China
[3] Univ Chinese Acad Sci UCAS, Beijing 100049, Peoples R China
[4] Zhengzhou Univ, Coll Chem, Zhengzhou 450001, Peoples R China
[5] Chinese Acad Sci, GPL Photon Lab, State Key Lab Appl Opt, Changchun Inst Opt Fine Mech & Phys, Changchun 130033, Peoples R China
[6] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore
关键词
color cognition; component engineering; microwire arrays; perovskites; photodetectors; NANOWIRES;
D O I
10.1002/adfm.202214094
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Color-cognitive detection plays an important role in many developing applications such as optical sensing, high-solution imaging, wearable biometric monitoring, and human visual cognitive system. Although color-cognitive devices have been demonstrated, the large size, complex manufacturing, high cost, and non-flexible processing impede their applications for distinguishing color information. Herein, gradient bandgap-tunable perovskite microwire arrays with excellent crystallinity and pure crystallographic orientation are realized by the synergy of the capillary-bridge assembly method and mild component engineering processing, yielding high-performance integrated color-cognitive devices with the spectral resolution of 14 nm ranging from 405 nm to 760 nm, responsivities over 10(3) A W-1, and detectivities over 10(15) Jones. Furthermore, the integrated flexible color-cognitive devices are demonstrated for accurately recognizing similar colors, which can be applied in color blindness correction. The efficient color recognition performances, together with the flexible processing, open new opportunities for the on-chip integration of wearable devices based on microwire arrays.
引用
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页数:10
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