Paths From Aerosol Particles to Activation and Cloud Droplets in Shallow Cumulus Clouds: The Roles of Entrainment and Supersaturation Fluctuations

The activation of aerosol particles and its contribution to cloud droplet size distributions in shallow cumulus clouds are investigated by analyzing the cloud field simulation results using a Lagrangian cloud model coupled with large eddy simulation, which allows explicit simulations of the activation and tracking of each super-droplet. Analysis is focused on the differences in activations for aerosol particles following central updraft from a cloud base (CB) and particles entrained above the cloud base (EA). Time series of various variables following individual particles confirm the distinctive nature of CB and EA activation. Strong supersaturation fluctuations induced by entrainment and turbulent mixing at cloud edges cause most EA particles to be deactivated soon after activation, substantially limiting their lifetime and growth relative to CB particles. Most net activation-the difference between activation and deactivation-occurs at the cloud base and vanishes aloft. Cloud droplet activation spectra follow the theoretical prediction at high supersaturation conditions, although the proportional constant is smaller because of particle deactivation. The spectra deviate from the theoretical prediction at low supersaturation conditions since they are affected by the transport of the CB particles activated elsewhere.