Chiral electroluminescence from thin-film perovskite metacavities

被引:15
作者
Kim, Seongheon [1 ]
An, Soo-Chan [1 ]
Kim, Younggon [1 ]
Shin, Yun Seop [2 ]
Antonov, Alexander A. [3 ]
Seo, In Cheol [1 ]
Woo, Byung Hoon [1 ]
Lim, Yeonsoo [1 ]
Gorkunov, Maxim V. [3 ,4 ]
Kivshar, Yuri S. [5 ]
Kim, Jin Young [2 ,6 ]
Jun, Young Chul [1 ,7 ]
机构
[1] Ulsan Natl Inst Sci & Technol UNIST, Dept Mat Sci & Engn, Ulsan 44919, South Korea
[2] Ulsan Natl Inst Sci & Technol UNIST, Sch Energy & Chem Engn, Ulsan 44919, South Korea
[3] Russian Acad Sci, Fed Sci Res Ctr Crystallog & Photon, Shubnikov Inst Crystallog, Moscow 119333, Russia
[4] Natl Res Nucl Univ, Moscow Engn Phys Inst, MEPhI, Moscow 115409, Russia
[5] Australian Natl Univ, Nonlinear Phys Ctr, Res Sch Phys, Canberra, ACT 2601, Australia
[6] Ulsan Natl Inst Sci & Technol UNIST, Grad Grad Sch Carbon Neutral, Ulsan 44919, South Korea
[7] Ulsan Natl Inst Sci & Technol UNIST, Grad Sch Semicond Mat & Devices Engn, Ulsan 44919, South Korea
基金
澳大利亚研究理事会; 新加坡国家研究基金会; 俄罗斯科学基金会;
关键词
LIGHT-EMITTING DIODE; METAMATERIAL; EMISSION;
D O I
10.1126/sciadv.adh0414
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Chiral light sources realized in ultracompact device platforms are highly desirable for various applications. Among active media used for thin-film emission devices, lead-halide perovskites have been extensively studied for photoluminescence due to their exceptional properties. However, up to date, there have been no demonstrations of chiral electroluminescence with a substantial degree of circular polarization (DCP) based on perovskite materials, being critical for the development of practical devices. Here, we propose a concept of chiral light sources based on a thin-film perovskite metacavity and experimentally demonstrate chiral electroluminescence with a peak DCP approaching 0.38. We design a metacavity created by a metal and a dielectric metasurface supporting photonic eigenstates with a close-to-maximum chiral response. Chiral cavity modes facilitate asymmetric electroluminescence of pairs of left and right circularly polarized waves propagating in the opposite oblique directions. The proposed ultracompact light sources are especially advantageous for many applications requiring chiral light beams of both helicities.
引用
收藏
页数:10
相关论文
共 50 条
  • [21] Circularly Polarized Electroluminescence From Chiral Manganese(II) Complexes
    Huo, Zhong-Zhong
    Wang, Yu
    Yang, Bo
    Liang, Jia-Qi
    Hong, Xian-Fang
    An, Qi
    Yuan, Li
    Ma, Huili
    Zuo, Jing-Lin
    Zheng, You-Xuan
    ADVANCED OPTICAL MATERIALS, 2025, 13 (08):
  • [22] Adaptive holographic pumping of thin-film organic lasers
    Wood, Simon M.
    Mavrogordatos, Themistoklis K.
    Morris, Stephen M.
    Hands, Philip J. W.
    Castles, Flynn
    Gardiner, Damian J.
    Atkinson, Katie L.
    Coles, Harry J.
    Wilkinson, Timothy D.
    OPTICS LETTERS, 2013, 38 (21) : 4483 - 4486
  • [23] Efficient and Tunable Electroluminescence from In Situ Synthesized Perovskite Quantum Dots
    Yu, Hongling
    Wang, Heyong
    Zhang, Jiangbin
    Lu, Jun
    Yuan, Zhongcheng
    Xu, Weidong
    Hultman, Lars
    Bakulin, Artem A.
    Friend, Richard H.
    Wang, Jianpu
    Liu, Xiao-Ke
    Gao, Feng
    SMALL, 2019, 15 (08)
  • [24] Model of electron transport in cell of a thin-film vacuum nanotriode
    Gallyamov, Z. R.
    Nikiforov, K. A.
    1ST INTERNATIONAL SCHOOL AND CONFERENCE SAINT-PETERSBURG OPEN 2014 ON OPTOELECTRONICS, PHOTONICS, ENGINEERING AND NANOSTRUCTURES, 2014, 541
  • [25] Dynamic carbon mitigation analysis: the role of thin-film photovoltaics
    Emmott, C. J. M.
    Ekins-Daukes, N. J.
    Nelson, J.
    ENERGY & ENVIRONMENTAL SCIENCE, 2014, 7 (06) : 1810 - 1818
  • [26] Room-temperature lasing from fluorene thin-film crystals densely doped with anthracene
    Aoki-Matsumoto, Tamao
    Mizuno, Hitoshi
    Ichida, Masao
    Ando, Hiroaki
    Hirai, Takeshi
    Mizuno, Ken-ichi
    OPTICS LETTERS, 2012, 37 (23) : 4880 - 4882
  • [27] Probing thin-film morphology of conjugated polymers by Raman spectroscopy
    Winfield, Jessica M.
    Donley, Carrie L.
    Friend, Richard H.
    Kim, Ji-Seon
    JOURNAL OF APPLIED PHYSICS, 2010, 107 (02)
  • [28] Design of thin-film photonic crystals with complete photonic bandgap
    Park, Se-Young
    Kim, Heungjoon
    Song, Bong-Shik
    OPTICS EXPRESS, 2018, 26 (22): : 29521 - 29526
  • [29] Directional Light Extraction from Photonic Crystal Thin-film GaN Light-Emitting Diodes
    Chao, Chia-Hsin
    Lai, Chun-Feng
    Kuo, Hao-Chung
    Yeh, Wen-Yung
    2009 LASERS & ELECTRO-OPTICS & THE PACIFIC RIM CONFERENCE ON LASERS AND ELECTRO-OPTICS, VOLS 1 AND 2, 2009, : 1289 - +
  • [30] Control of fluorescence enhancement and directionality upon excitations in a thin-film system
    Chen, Xingxing
    Chen, Yu-Hui
    Qiu, Min
    Blaikie, Richard J.
    Ding, Boyang
    PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS, 2015, 252 (10): : 2222 - 2229