Bubble-propelled micromotors for ammonia generation

被引:4
作者
Campos, Rebeca Ferrer [1 ]
Bachimanchi, Harshith [2 ]
Volpe, Giovanni [2 ]
Villa, Katherine [1 ]
机构
[1] Inst Chem Res Catalonia ICIQ, Av Paisos Catalans 16, E-43007 Tarragona, Spain
[2] Univ Gothenburg, Dept Phys, Origovagen 6B, S-41296 Gothenburg, Sweden
基金
欧洲研究理事会;
关键词
CATALYTIC MICROMOTORS; REMOVAL; LACCASE; POLLUTANTS; UREA;
D O I
10.1039/d3nr03804a
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Micromotors have emerged as promising tools for environmental remediation, thanks to their ability to autonomously navigate and perform specific tasks at the microscale. In this study, we present the development of MnO2 tubular micromotors modified with laccase for enhanced oxidation of organic pollutants by providing an additional oxidative catalytic pathway for pollutant removal. These modified micromotors exhibit efficient ammonia generation through the catalytic decomposition of urea, suggesting their potential application in the field of green energy generation. Compared to bare micromotors, the MnO2 micromotors modified with laccase exhibit a 20% increase in rhodamine B degradation. Moreover, the generation of ammonia increased from 2 to 31 ppm in only 15 min, evidencing their high catalytic activity. To enable precise tracking of the micromotors and measurement of their speed, a deep-learning-based tracking system was developed. Overall, this work expands the potential applicability of bio-catalytic tubular micromotors in the energy field. Here, we introduce self-propelled biocatalytic micromotors for simultaneous organic pollutant removal and green energy generation. The study demonstrates remarkable results, showcasing the potential to generate ammonia from wastewater in short time.
引用
收藏
页码:15785 / 15793
页数:9
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