TiO2/Activated Carbon/2D Selenides Composite Photocatalysts for Industrial Wastewater Treatment

被引:7
作者
Ahmad, Shehzad [1 ]
Tahir, Muhammad Suleman [2 ,3 ]
Kamal, Ghulam Mustafa [1 ,4 ]
Zhang, Xu [5 ,6 ,7 ]
Nazir, Saima [4 ,8 ]
Tahir, Muhammad Bilal [9 ]
Jiang, Bin [5 ,6 ,7 ]
Safdar, Muhammad [1 ]
机构
[1] Khwaja Fareed Univ Engn & Informat Technol, Inst Chem, Rahim Yar Khan 64200, Pakistan
[2] Khwaja Fareed Univ Engn & Informat Technol, Inst Chem & Environm Engn, Rahim Yar Khan 64200, Pakistan
[3] Univ Gujrat, Dept Chem Engn, Gujrat 50700, Pakistan
[4] Khwaja Fareed Univ Engn & Informat Technol, Inst Hlth Sci, Rahim Yar Khan 64200, Pakistan
[5] Opt Valley Lab, Wuhan 430074, Peoples R China
[6] Chinese Acad Sci, Wuhan Inst Phys & Math, Innovat Acad Precis Measurement Sci & Technol, Natl Ctr Magnet Resonance Wuhan,Key Lab Magnet Res, Wuhan 430074, Peoples R China
[7] Huazhong Univ Sci & Technol, Wuhan Natl Lab Optoelect, Wuhan 430071, Peoples R China
[8] Univ Gujrat, Nawaz Sharif Med Coll, Gujrat 50700, Pakistan
[9] Khwaja Fareed Univ Engn & Informat Technol, Inst Phys, Rahim Yar Khan 64200, Pakistan
基金
中国国家自然科学基金;
关键词
TiO(2)activated carbon; 2D selenides; photocatalyst; wastewater treatment; GRAPHENE SAND COMPOSITE; TIO2; NANOPARTICLES; OPTICAL-PROPERTIES; DOPED TIO2; DEGRADATION; NANOTECHNOLOGY; MOS2; DYE; OXYTETRACYCLINE; MINERALIZATION;
D O I
10.3390/w15091788
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Even in the 21st century, water contamination has been a big problem and industrial processes are to be blamed for polluted water supplies. The use of sunlight in the process of photocatalysis is an efficientway to purifywastewater. Composites of TiO2/activated carbon/two-dimensional selenides performed better than either of the individual material or binary composites for this application. A straightforward hydrothermal technique was employed in the synthesis of photocatalysts. The synthesized photocatalytic composites were verified with the help of UV-Visible spectroscopy, FTIR, XRD, and SEM. The heterostructures absorbed nearly all of the sun's UV and visible light. These photons are then converted into usable reducing electrons and oxidizing species such as O-center dot(2) and OH center dot to decompose organic pollutants from industrial wastewater. Since there were additional pathways available for charge transfer along with several active edge sites, the composite photocatalysts are proven more active than individual TiO2 and 2D MoSe2 components. With the help of a cascadedriven mechanism of electrons, these channels can transmit more charges than single-component heterojunctions. The results provided a realistic method for developing photocatalyst composites powered by solar light for use in industrial wastewater treatment. Results of degradation of methylene blue suggest that the synthesized composites possess better photocatalytic activity. This enhanced photocatalytic activity is not limited to organic dyes. Other hazardous organic pollutants present in industrial wastewater can be decomposed by using this approach.
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页数:22
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