Recent progress on covalent organic frameworks for photocatalytic hydrogen generation via water splitting

被引:21
作者
Zhu, Shan-Shan [1 ,2 ]
Zhang, Zhenwei [1 ,2 ]
Li, Zhongping [1 ,2 ]
Liu, Xiaoming [1 ,2 ]
机构
[1] Jilin Univ, Coll Chem, Changchun 130012, Peoples R China
[2] Ulsan Natl Inst Sci & Technol UNIST, Ctr Dimens Controllable Organ Frameworks, Sch Energy & Chem Engn, Ulsan 44919, South Korea
基金
中国国家自然科学基金;
关键词
GRAPHITIC CARBON NITRIDE; EXCITON BINDING-ENERGIES; H-2; EVOLUTION; FACILE SYNTHESIS; NANOMATERIALS; CRYSTALLINE; HYBRID; HETEROJUNCTIONS; CONSTRUCTION; COCATALYSTS;
D O I
10.1039/d3qm00965c
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Currently, the excessive consumption of conventional fossil fuels has caused the energy crisis and environmental pollution. Efficient solar-driven photocatalysts for the hydrogen evolution reaction (HER) are essential to facilitate future hydrogen-powered technologies. Covalent organic frameworks (COFs) with permanent porosity, long-range order and rigid backbones offer a promising material platform to address the global energy need. In this review, we focus on different strategies to improve the performance of COF-based photocatalysts and the factors involved in photocatalytic water splitting for hydrogen production. Finally, an overview on the prospects and challenges in the rational design of COF-based photocatalysts in the field of photocatalysis is outlined.
引用
收藏
页码:1513 / 1535
页数:23
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