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Piezo-photocatalytic reduction of toxic Cr(VI) ions based on MoS2 nanoflowers
被引:18
|作者:
Li, Xiu
[1
]
Ren, Zeqian
[1
]
Zhang, Qiwei
[1
]
Guo, Lixia
[1
]
Wu, Jizhou
[1
,2
]
Li, Yuqing
[1
,2
]
Liu, Wenliang
[1
,2
]
Li, Peng
[1
]
Fu, Yongming
[1
]
Ma, Jie
[1
,2
]
机构:
[1] Shanxi Univ, Inst Laser Spect, Sch Phys & Elect Engn, State Key Lab Quantum Opt & Quantum Opt Devices, Taiyuan 030006, Peoples R China
[2] Shanxi Univ, Collaborat Innovat Ctr Extreme Opt, Taiyuan 030006, Peoples R China
基金:
国家重点研发计划;
俄罗斯基础研究基金会;
中国国家自然科学基金;
关键词:
Nanoparticles;
Piezoelectric materials;
Cr6+ reduction;
Piezo-photocatalysis;
MoS2;
nanoflower;
D O I:
10.1016/j.matlet.2022.133564
中图分类号:
T [工业技术];
学科分类号:
08 ;
摘要:
The reduction of Cr6+ is very important for sewage treatment. Here, a strategy is proposed for the highly efficient reduction of Cr6+ by co-utilizing the photocatalysis and piezoelectric effect of MoS2 nanoflowers. Under both solar-irradiation (300 W Xe lamp) and ultrasonication, the Cr6+ removal rate catalyzed by few-layer MoS2 nanoflowers (10 mg) increases with increasing ultrasonication power, and a maximum of 96.22 % is achieved under solar irradiation and ultrasonication (100 W) for 20 min, similar to 3.65-fold of that under only solar irradiation. The fast Cr6+ removal rate can be ascribed to the synergistic effect of light induced reduction effect and ultrasound induced piezoelectric field. This work explores a new approach for highly efficient Cr6+ removal.
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