A leap by the rise of solid-state electrolytes for Li-air batteries

被引:33
作者
Pan, Kecheng [1 ]
Li, Minghui [1 ]
Wang, Weicheng [1 ]
Xing, Shuochao [1 ]
Dou, Yaying [1 ]
Gao, Shasha [2 ]
Zhang, Zhang [1 ,3 ]
Zhou, Zhen [1 ]
机构
[1] Zhengzhou Univ, Sch Chem Engn, Interdisciplinary Res Ctr Sustainable Energy Sci &, Zhengzhou 450001, Peoples R China
[2] Xinyang Normal Univ, Dept Phys & Elect Engn, Key Lab Microelect & Energy Henan Prov, Xinyang 464000, Peoples R China
[3] Nankai Univ, Coll Chem, Key Lab Adv Energy Mat Chem, Minist Educ, Tianjin 300071, Peoples R China
关键词
Solid-state Li-air batteries; Solid-state electrolytes; Interfacial compatibility and verifiability; LITHIUM-OXYGEN BATTERY; LONG-CYCLE-LIFE; POLYMER ELECTROLYTES; LI-O-2; BATTERY; LI-CO2; TEMPERATURE; PERFORMANCE;
D O I
10.1016/j.gee.2023.02.010
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Li-air batteries have attracted extensive attention because of their ultrahigh theoretical energy density. However, the potential safety hazard of flammable organic liquid electrolytes hinders their practical applications. Replacing liquid electrolytes with solidstate electrolytes (SSEs) is expected to fundamentally overcome the safety issues. In this work, we focus on the development and challenge of solid-stateLi-air batteries (SSLABs). The rise of different types of SSEs, interfacial compatibility and verifiability in SSLABs are presented. The corresponding strategies and prospects of SSLABs are also proposed. In particular, combining machine learning method with experiment and in situ (or operando) techniques is imperative to accelerate the development of SSLABs. (c) 2023 Institute of Process Engineering, Chinese Academy of Sciences. Publishing services by Elsevier B.V. on behalf of KeAi Communications Co., Ltd. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
引用
收藏
页码:939 / 944
页数:6
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