Experimental study on the performance of a highly efficient NE-1 absorbent for CO2 capture

被引:0
作者
Huang, Chenzhi [1 ,6 ]
Cao, Yongda [1 ]
Li, Yaxin [1 ]
Li, Qi [2 ]
Liu, Qiang [3 ]
Xia, Lin [4 ]
Peng, Xiujun [1 ]
Yue, Hairong [5 ]
机构
[1] PetroChina Southwest Oil & Gasfield Co, Res Inst Nat Gas Technol, Chengdu, Sichuan, Peoples R China
[2] PetroChina Southwest Oil & Gasfield Co, Chengdu, Sichuan, Peoples R China
[3] PetroChina Southwest Oil & Gasfield Co, New Energy Div, Chengdu, Sichuan, Peoples R China
[4] PetroChina Southwest Oil & Gasfield Co, Nat Gas Purificat Plant Gen, Chongqing, Peoples R China
[5] Sichuan Univ, Sch Chem Engn, Chengdu, Sichuan, Peoples R China
[6] PetroChina Southwest Oil & Gasfield Co, Res Inst Nat Gas Technol, Chengdu 610213, Sichuan, Peoples R China
关键词
CO2; capture; liquid amine; absorption; corrosion inhibitor; thermal degradation; DESORPTION; SOLVENTS; ALKANOLAMINE; ABSORPTION; CORROSION; ACID; MEA;
D O I
10.1002/ghg.2272
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
CO2 capture by absorption and stripping with aqueous amine is a well-understood and widely used technology. However, drawbacks still exist in the practical applications, such as high energy consumption and easy degradation of the absorbents during the desorption process. In this paper, a novel NE-1 absorbent was developed, and its suitable operating conditions were determined: concentration (45 wt.%), absorption temperature (40 degrees C), and desorption temperature (100 degrees C). The NE-1 absorbent exhibits a high CO2 absorption capacity of 3.73 mol/kg, 1.33 times that of 30% monoethanolamine (MEA). After optimizing with carbamide as a corrosion inhibitor, 45% NE-1a1 may attain an effective CO2 capacity of 2.5 mol/kg and over 70% desorption rate in five cycles, demonstrating excellent cycling stability performance. The research results have significant implications for developing an efficient and stable commercial carbon capture solvent and promoting the development of carbon reduction technologies. (c) 2024 Society of Chemical Industry and John Wiley & Sons, Ltd.
引用
收藏
页码:442 / 455
页数:14
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