Deep learning;
LIBS spectroscopy;
Jewelry rock;
Convolutional LSTM;
Chemometrics;
LIBS;
D O I:
10.1038/s41598-024-55502-x
中图分类号:
O [数理科学和化学];
P [天文学、地球科学];
Q [生物科学];
N [自然科学总论];
学科分类号:
07 ;
0710 ;
09 ;
摘要:
In this study, the deep learning algorithm of Convolutional Neural Network long short-term memory (CNN-LSTM) is used to classify various jewelry rocks such as agate, turquoise, calcites, and azure from various historical periods and styles related to Shahr-e Sokhteh. Here, the CNN-LSTM architecture includes utilizing CNN layers for the extraction of features from input data mixed with LSTMs for supporting sequence forecasting. It should be mentioned that interpretable deep learning-assisted laser induced breakdown spectroscopy helped achieve excellent performance. For the first time, this paper interprets the Convolutional LSTM effectiveness layer by layer in self-adaptively obtaining LIBS features and the quantitative data of major chemical elements in jewelry rocks. Moreover, Lasso method is applied on data as a factor for investigation of interoperability. The results demonstrated that LIBS can be essentially combined with a deep learning algorithm for the classification of different jewelry songs. The proposed methodology yielded high accuracy, confirming the effectiveness and suitability of the approach in the discrimination process.
机构:
CNR, Res Area, Appl & Laser Spect Lab, Inst Chem Organometall Cpds, Via G Moruzzi 1, I-56124 Pisa, ItalyUniv Pisa, Dept Chem & Ind Chem, Via G Moruzzi 13, I-56124 Pisa, Italy
Lorenzetti, Giulia
Pagnotta, Stefano
论文数: 0引用数: 0
h-index: 0
机构:
CNR, Res Area, Appl & Laser Spect Lab, Inst Chem Organometall Cpds, Via G Moruzzi 1, I-56124 Pisa, Italy
Univ Pisa, Dept Earth Sci, Via Santa Maria 53, I-56126 Pisa, ItalyUniv Pisa, Dept Chem & Ind Chem, Via G Moruzzi 13, I-56124 Pisa, Italy
Pagnotta, Stefano
Poggialini, Francesco
论文数: 0引用数: 0
h-index: 0
机构:
CNR, Res Area, Appl & Laser Spect Lab, Inst Chem Organometall Cpds, Via G Moruzzi 1, I-56124 Pisa, Italy
Scuola Normale Super Pisa, Piazza Cavalieri 7, I-56126 Pisa, ItalyUniv Pisa, Dept Chem & Ind Chem, Via G Moruzzi 13, I-56124 Pisa, Italy
Poggialini, Francesco
Palleschi, Vincenzo
论文数: 0引用数: 0
h-index: 0
机构:
CNR, Res Area, Appl & Laser Spect Lab, Inst Chem Organometall Cpds, Via G Moruzzi 1, I-56124 Pisa, ItalyUniv Pisa, Dept Chem & Ind Chem, Via G Moruzzi 13, I-56124 Pisa, Italy
机构:
Chinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chinese Acad Sci, Key Lab Networked Control Syst, Shenyang 110016, Peoples R China
Chinese Acad Sci, Inst Robot, Shenyang 110169, Peoples R China
Chinese Acad Sci, Inst Intelligent Mfg, Shenyang 110169, Peoples R China
Univ Chinese Acad Sci, Beijing 100049, Peoples R ChinaChinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chen, Tong
Sun, Lanxiang
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chinese Acad Sci, Key Lab Networked Control Syst, Shenyang 110016, Peoples R China
Chinese Acad Sci, Inst Robot, Shenyang 110169, Peoples R China
Chinese Acad Sci, Inst Intelligent Mfg, Shenyang 110169, Peoples R ChinaChinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Sun, Lanxiang
Yu, Haibin
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chinese Acad Sci, Key Lab Networked Control Syst, Shenyang 110016, Peoples R China
Chinese Acad Sci, Inst Robot, Shenyang 110169, Peoples R China
Chinese Acad Sci, Inst Intelligent Mfg, Shenyang 110169, Peoples R ChinaChinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Yu, Haibin
Wang, Wei
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chinese Acad Sci, Key Lab Networked Control Syst, Shenyang 110016, Peoples R China
Chinese Acad Sci, Inst Robot, Shenyang 110169, Peoples R China
Chinese Acad Sci, Inst Intelligent Mfg, Shenyang 110169, Peoples R China
Univ Chinese Acad Sci, Beijing 100049, Peoples R ChinaChinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Wang, Wei
Qi, Lifeng
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chinese Acad Sci, Key Lab Networked Control Syst, Shenyang 110016, Peoples R China
Chinese Acad Sci, Inst Robot, Shenyang 110169, Peoples R China
Chinese Acad Sci, Inst Intelligent Mfg, Shenyang 110169, Peoples R ChinaChinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Qi, Lifeng
Zhang, Peng
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chinese Acad Sci, Key Lab Networked Control Syst, Shenyang 110016, Peoples R China
Chinese Acad Sci, Inst Robot, Shenyang 110169, Peoples R China
Chinese Acad Sci, Inst Intelligent Mfg, Shenyang 110169, Peoples R ChinaChinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Zhang, Peng
Zeng, Peng
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chinese Acad Sci, Key Lab Networked Control Syst, Shenyang 110016, Peoples R China
Chinese Acad Sci, Inst Robot, Shenyang 110169, Peoples R China
Chinese Acad Sci, Inst Intelligent Mfg, Shenyang 110169, Peoples R ChinaChinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
机构:
Univ Bordeaux, LOMA, UMR 5798, F-33400 Talence, France
CNRS, LOMA, UMR 5798, F-33400 Talence, FranceUniv Bordeaux, LOMA, UMR 5798, F-33400 Talence, France
Canioni, L.
Bousquet, B.
论文数: 0引用数: 0
h-index: 0
机构:
Univ Bordeaux, LOMA, UMR 5798, F-33400 Talence, France
CNRS, LOMA, UMR 5798, F-33400 Talence, FranceUniv Bordeaux, LOMA, UMR 5798, F-33400 Talence, France
机构:
CNR, Res Area, Appl & Laser Spect Lab, Inst Chem Organometall Cpds, Via G Moruzzi 1, I-56124 Pisa, ItalyUniv Pisa, Dept Chem & Ind Chem, Via G Moruzzi 13, I-56124 Pisa, Italy
Lorenzetti, Giulia
Pagnotta, Stefano
论文数: 0引用数: 0
h-index: 0
机构:
CNR, Res Area, Appl & Laser Spect Lab, Inst Chem Organometall Cpds, Via G Moruzzi 1, I-56124 Pisa, Italy
Univ Pisa, Dept Earth Sci, Via Santa Maria 53, I-56126 Pisa, ItalyUniv Pisa, Dept Chem & Ind Chem, Via G Moruzzi 13, I-56124 Pisa, Italy
Pagnotta, Stefano
Poggialini, Francesco
论文数: 0引用数: 0
h-index: 0
机构:
CNR, Res Area, Appl & Laser Spect Lab, Inst Chem Organometall Cpds, Via G Moruzzi 1, I-56124 Pisa, Italy
Scuola Normale Super Pisa, Piazza Cavalieri 7, I-56126 Pisa, ItalyUniv Pisa, Dept Chem & Ind Chem, Via G Moruzzi 13, I-56124 Pisa, Italy
Poggialini, Francesco
Palleschi, Vincenzo
论文数: 0引用数: 0
h-index: 0
机构:
CNR, Res Area, Appl & Laser Spect Lab, Inst Chem Organometall Cpds, Via G Moruzzi 1, I-56124 Pisa, ItalyUniv Pisa, Dept Chem & Ind Chem, Via G Moruzzi 13, I-56124 Pisa, Italy
机构:
Chinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chinese Acad Sci, Key Lab Networked Control Syst, Shenyang 110016, Peoples R China
Chinese Acad Sci, Inst Robot, Shenyang 110169, Peoples R China
Chinese Acad Sci, Inst Intelligent Mfg, Shenyang 110169, Peoples R China
Univ Chinese Acad Sci, Beijing 100049, Peoples R ChinaChinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chen, Tong
Sun, Lanxiang
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chinese Acad Sci, Key Lab Networked Control Syst, Shenyang 110016, Peoples R China
Chinese Acad Sci, Inst Robot, Shenyang 110169, Peoples R China
Chinese Acad Sci, Inst Intelligent Mfg, Shenyang 110169, Peoples R ChinaChinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Sun, Lanxiang
Yu, Haibin
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chinese Acad Sci, Key Lab Networked Control Syst, Shenyang 110016, Peoples R China
Chinese Acad Sci, Inst Robot, Shenyang 110169, Peoples R China
Chinese Acad Sci, Inst Intelligent Mfg, Shenyang 110169, Peoples R ChinaChinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Yu, Haibin
Wang, Wei
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chinese Acad Sci, Key Lab Networked Control Syst, Shenyang 110016, Peoples R China
Chinese Acad Sci, Inst Robot, Shenyang 110169, Peoples R China
Chinese Acad Sci, Inst Intelligent Mfg, Shenyang 110169, Peoples R China
Univ Chinese Acad Sci, Beijing 100049, Peoples R ChinaChinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Wang, Wei
Qi, Lifeng
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chinese Acad Sci, Key Lab Networked Control Syst, Shenyang 110016, Peoples R China
Chinese Acad Sci, Inst Robot, Shenyang 110169, Peoples R China
Chinese Acad Sci, Inst Intelligent Mfg, Shenyang 110169, Peoples R ChinaChinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Qi, Lifeng
Zhang, Peng
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chinese Acad Sci, Key Lab Networked Control Syst, Shenyang 110016, Peoples R China
Chinese Acad Sci, Inst Robot, Shenyang 110169, Peoples R China
Chinese Acad Sci, Inst Intelligent Mfg, Shenyang 110169, Peoples R ChinaChinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Zhang, Peng
Zeng, Peng
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
Chinese Acad Sci, Key Lab Networked Control Syst, Shenyang 110016, Peoples R China
Chinese Acad Sci, Inst Robot, Shenyang 110169, Peoples R China
Chinese Acad Sci, Inst Intelligent Mfg, Shenyang 110169, Peoples R ChinaChinese Acad Sci, Shenyang Inst Automat, State Key Lab Robot, Shenyang 110016, Peoples R China
机构:
Univ Bordeaux, LOMA, UMR 5798, F-33400 Talence, France
CNRS, LOMA, UMR 5798, F-33400 Talence, FranceUniv Bordeaux, LOMA, UMR 5798, F-33400 Talence, France
Canioni, L.
Bousquet, B.
论文数: 0引用数: 0
h-index: 0
机构:
Univ Bordeaux, LOMA, UMR 5798, F-33400 Talence, France
CNRS, LOMA, UMR 5798, F-33400 Talence, FranceUniv Bordeaux, LOMA, UMR 5798, F-33400 Talence, France