Tar removal from the producer gas of a small scale downdraft gasifier using a fatty acid based, wet packed-bed scrubber

被引:3
作者
Lotfi, Samira [1 ,2 ]
Ma, Weiguo [1 ]
Austin, Kevin [1 ]
Luque, Luis [1 ]
Littlejohns, Jennifer V. [1 ]
Butler, James [1 ]
机构
[1] Natl Res Council Canada, Energy Min & Environm, Ottawa, ON, Canada
[2] Natl Res Council Canada, Energy Min & Environm, M-12 Montreal Rd, Ottawa, ON K1A 0R6, Canada
关键词
gasification; oil; packed-bed; tar removal; trickle bed; waste; wet packed-bed; wood chips; BIOMASS PYROLYSIS; VEGETABLE-OIL; TECHNOLOGIES; PERFORMANCE; ELIMINATION; ABSORPTION; REDUCTION; SYSTEM;
D O I
10.1002/cjce.25116
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Small scale gasification combined heat and power (CHP) systems offer an alternative to diesel fuelled generators for power generation in remote communities and industrial sites. Tar and particulates in the producer-gas can damage the internal combustion engine generator and increase operation and maintenance costs. In this work, we present a novel trickle-bed scrubber using filtered waste cooking oil as a cost effective and easy-to-operate gas clean-up method for a small CHP system. The performance of the trickle-bed scrubber was compared against a packed-bed filter utilizing woodchips in a 20 kW(th) downdraft gasifier. Used-cooking oil was selected as the solvent and woodchips as the bed-material as these are readily available, inexpensive, and can be recycled in the gasifier as fuel. A woodchip packed-bed filter reduced the tar and particulate matter (PM) in the producer gas from gasification of spruce chips (11% moisture) from 1.6 to 1.4 g/Nm(3) and from 0.16 to 0.087 g/Nm(3) respectively. The trickle-bed scrubber was able to reduce the tar and PM in the producer gas from gasification of pinewood (8% moisture) from 1.38 to 0.28 g/Nm(3), and 0.209 to 0.082 g/Nm(3), respectively. Tar and PM removal efficiency improved by 60% and 29% respectively. Components such as benzene, toluene, naphthalene, and biphenylene were the major tar components. After passing the trickle-bed, most tar was removed, with a preference for removal of multi-ringed aromatics and gravimetric tars. Parameters such as the tar and particulate concentration, feedstock moisture content, and feedstock source affect the performance of the gas clean-up system.
引用
收藏
页码:607 / 621
页数:15
相关论文
共 41 条
[11]   Research progress of hot gas filtration, desulphurization and HCl removal in coal-derived fuel gas: A review [J].
Dou, Binlin ;
Wang, Chao ;
Chen, Haisheng ;
Song, Yongchen ;
Xie, Baozheng ;
Xu, Yujie ;
Tan, Chunqing .
CHEMICAL ENGINEERING RESEARCH & DESIGN, 2012, 90 (11) :1901-1917
[12]   Ash Management Review-Applications of Biomass Bottom Ash [J].
James, Adrian K. ;
Thring, Ronald W. ;
Helle, Steve ;
Ghuman, Harpuneet S. .
ENERGIES, 2012, 5 (10) :3856-3873
[13]   Small Scale Gasification Application and Perspectives in Circular Economy [J].
Klavins, Maris ;
Bisters, Valdis ;
Burlakovs, Juris .
ENVIRONMENTAL AND CLIMATE TECHNOLOGIES, 2018, 22 (01) :42-54
[14]  
Le Coq L., EUCOMC 19 EUCHEMS C
[15]   Experimental Investigation of Bioenergy Production from Small-Scale Gasification of Landfill-Diverted Wood Wastes [J].
Littlejohns, Jennifer, V ;
Butler, James ;
Luque, Luis ;
Austin, Kevin .
WASTE AND BIOMASS VALORIZATION, 2020, 11 (12) :6885-6901
[16]  
Lotfi S, 2021, Petroleum & Petrochemical Engineering Journal, V5, P1, DOI [10.23880/ppej-16000271, 10.23880/ppej-16000271, DOI 10.23880/PPEJ-16000271]
[17]   Modeling as a Tool for the Optimal Design of a Downdraft Gasifier Operating on Waste Feedstock [J].
Lotfi, Samira ;
Littlejohns, Jennifer ;
Austin, Kevin ;
Luque, Luis .
WASTE AND BIOMASS VALORIZATION, 2021, 12 (12) :6569-6589
[18]   A wet packed-bed scrubber for removing tar from biomass producer gas [J].
Lotfi, Samira ;
Ma, Weiguo ;
Austin, Kevin ;
Kumar, Ashwani .
FUEL PROCESSING TECHNOLOGY, 2019, 193 :197-203
[19]   Studies for removal of tar from producer gas in small scale biomass gasifiers using biodiesel [J].
Madav, Vasudeva ;
Das, Darpan ;
Kumar, Manish ;
Surwade, Manoj ;
Parikh, P. P. ;
Sethi, Virendra .
BIOMASS & BIOENERGY, 2019, 123 :123-133
[20]  
Milne T., 1998, Biomass Gasifier "Tars": Their Nature, Formation and Conversion, DOI DOI 10.2172/3726