Design of ternary CeO2/Fe2O3/reduced graphene oxide-based hybrid nanocomposite for superior photocatalytic degradation material for organic dyes

被引:16
作者
Gomathi, A. [1 ]
Prabhuraj, T. [1 ]
Gokilapriya, S. [1 ]
Vasanthi, G. [1 ]
Maadeswaran, P. [1 ]
Kumar, K. A. Ramesh [2 ]
机构
[1] Periyar Univ, Dept Energy Sci & Technol, Adv Nanomat & Energy Res Lab, Salem 636011, India
[2] Periyar Univ, Dept Energy Sci & Technol, Adv Bioenergy & Biofuels Res Lab, Salem 636011, India
关键词
CeO; 2; Fe; O; 3; r-GO hybrid composite; Organic dyes; Photocatalytic dye degradation efficiency; VISIBLE-LIGHT-DRIVEN; TEXTILE DYE; COMPOSITE; TIO2; PERFORMANCE; REMOVAL; TITANIA;
D O I
10.1016/j.dyepig.2023.111473
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
Green energy and environmental preservation are becoming two foremost concerns in the human society. A successful strategy for addressing the issue of environmental pollution the photocatalytic application was helped to breakdown the harmful substances and sterilization of microorganisms in the presence of catalyst and sunlight. Herein, we introduced a serious of ternary CeO2/Fe2O3/r-GO based hybrid nanocomposite as an efficient catalyst for dye-degradation process. The effective catalyst was prepared via simple hydrothermal method assisted with annealing route. The hybrid catalyst was subjected to the XRD, FTIR, SEM and UV-DRS to estimate the structural and optical properties. Based on the study, the hybrid CeO2/Fe2O3/r-GO nanocomposite was exposed the brilliant absorption characteristics phenomena, and photocatalytic activities with remarkable stability. The methylene blue and methylene orange dye degradation activities were estimated using with the prepared hybrid nanocomposite. Fascinatingly, the hybrid CeO2/Fe2O3/r-GO catalyst was delivered the 90% and 86% dye-degradation result in the methylene blue and orange dyes under the UV light irradiation. Additionally, CeO2/Fe2O3/r-GO composite was gratefully recycled for five photodegradation sequences without experiencing any substantial changes to its activity or crystalline characteristics. The improved photocatalytic activity of the CeO2/Fe2O3/r-GO catalyst was mainly permitted to the synergic effects of the heterojunctions in the interface. The study's goal is to provide a good understanding for designing a suitable visible-light-driven photocatalyst with acceptable environmental remediation.
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页数:13
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共 66 条
  • [1] Solution-processed CeO2/TiO2 nanocomposite as potent visible light photocatalyst for the degradation of bromophenol dye
    Ameen, Sadia
    Akhtar, M. Shaheer
    Seo, Hyung-Kee
    Shin, Hyung-Shik
    [J]. CHEMICAL ENGINEERING JOURNAL, 2014, 247 : 193 - 198
  • [2] Photoelectrochemical hybrid cell for unbiased CO2 reduction coupled to alcohol oxidation
    Anton-Garcia, Daniel
    Moore, Esther Edwardes
    Bajada, Mark A.
    Eisenschmidt, Annika
    Oliveira, Ana R.
    Pereira, Ines A. C.
    Warnan, Julien
    Reisner, Erwin
    [J]. NATURE SYNTHESIS, 2022, 1 (01): : 77 - 86
  • [3] Controllable synthesis of CeO2/g-C3N4 hybrid catalysts and its structural, optical and visible light photocatalytic activity
    Barathi, D.
    Rajalakshmi, N.
    Ranjith, R.
    Sangeetha, R.
    Meyvel, S.
    [J]. DIAMOND AND RELATED MATERIALS, 2021, 111
  • [4] Novel photocatalyst: Titania-coated magnetite. Activity and photodissolution
    Beydoun, D
    Amal, R
    Low, GKC
    McEvoy, S
    [J]. JOURNAL OF PHYSICAL CHEMISTRY B, 2000, 104 (18) : 4387 - 4396
  • [5] Synthesis and room-temperature ultraviolet photoluminesence properties of zirconia nanowires
    Cao, HQ
    Qiu, XQ
    Luo, B
    Liang, Y
    Zhang, YH
    Tan, RQ
    Zhao, MJ
    Zhu, QM
    [J]. ADVANCED FUNCTIONAL MATERIALS, 2004, 14 (03) : 243 - 246
  • [6] Photocatalytic activity under visible light of Fe-doped CeO2 nanoparticles synthesized by flame spray pyrolysis
    Channei, D.
    Inceesungvorn, B.
    Wetchakun, N.
    Phanichphant, S.
    Nakaruk, A.
    Koshy, P.
    Sorrell, C. C.
    [J]. CERAMICS INTERNATIONAL, 2013, 39 (03) : 3129 - 3134
  • [7] The preparation of coupled WO3/TiO2 photocatalyst by ball milling
    Chen, SF
    Chen, L
    Gao, S
    Cao, GY
    [J]. POWDER TECHNOLOGY, 2005, 160 (03) : 198 - 202
  • [8] Comprehensive review and future perspectives on the photocatalytic hydrogen production
    Corredor, Juan
    Rivero, Maria J.
    Rangel, Carmen M.
    Gloaguen, Frederic
    Ortiz, Inmaculada
    [J]. JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY, 2019, 94 (10) : 3049 - 3063
  • [9] Synthesis of the graphene-ZnTiO3 nanocomposite for solar light assisted photodegradation of methylene blue
    Gayathri, Shunmugiah
    Jayabal, Palanisamy
    Kottaisamy, Muniasamy
    Ramakrishnan, Veerabahu
    [J]. JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2015, 48 (41)
  • [10] Kinetic and adsorption study of acid dye removal using activated carbon
    Gomez, V.
    Larrechi, M. S.
    Callao, M. P.
    [J]. CHEMOSPHERE, 2007, 69 (07) : 1151 - 1158