Formation of Droplets of Shear-Thinning Non-Newtonian Fluids in Asymmetrical Parallelized Microchannels

被引:5
|
作者
Dong, Yanpeng [1 ]
Xiang, Xingyu [1 ]
Wang, Zhongdong [1 ]
Zhu, Chunying [1 ]
Ma, Youguang [1 ]
Fu, Taotao [1 ]
机构
[1] Tianjin Univ, Sch Chem Engn & Technol, State Key Lab Chem Engn, Tianjin 300072, Peoples R China
基金
中国国家自然科学基金;
关键词
RECTANGULAR MICROCHANNELS; BREAKUP DYNAMICS; PRESSURE-DROP; FLOW; HYDRODYNAMICS; MICROREACTOR; DESIGN;
D O I
10.1021/acs.langmuir.2c02736
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Fluids containing polymers are frequently utilized in the chemical industry and exhibit shear-thinning characteristics. The flow distribution of non-Newtonian fluids in parallelized microchannels is a key issue to be solved during numbering-up. Numbering-up means increasing the number of parallelized micro-channels. In this study, a high-speed camera is used to explore the distribution of fluid flow as well as the uniformity and stability of droplets in conceptual asymmetrical parallelized microchannels. Cyclohexane and carboxymethylcellulose sodium (CMC) aqueous solutions are used as the continuous phase and dispersed phase, respectively. The effects of fluctuation of pressure difference around the T-junction, the hydrodynamic resistance in microchannels, and the shear-thinning property of fluids on flow distribution and droplet formation are revealed. The uniformity and stability of droplets in microdevices with various cavity settings are compared, and an optimal configuration is proposed. Finally, prediction models for the flow distribution of shear-thinning fluids in asymmetrical parallelized microchannels are established.
引用
收藏
页码:2218 / 2232
页数:15
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