Pd oxide nanoparticles enhanced biomass driven N-doped carbon for hydrogen evolution reaction

被引：9

作者：

Li, Hongyu ^{[1
]}

机构：

[1] Guilin Univ Technol, Coll Chem & Bioengn, Guangxi Key Lab Electrochem & Magneto Chem Funct M, Guilin 541004, Peoples R China

来源：

CHEMICAL PHYSICS LETTERS | 2023年 / 815卷

基金：

中国国家自然科学基金;

关键词：

Biomass; Waste durian shell; Pd oxide nanoparticles; Electrocatalyst; Hydrogen evolution reaction (HER); COAL-DERIVED CARBON; ACTIVATED CARBON; OXYGEN REDUCTION; POROUS CARBON; HIGH-ENERGY; EFFICIENT; ELECTROCATALYSTS; NANOSHEETS; GRAPHENE; ARRAYS;

D O I：

10.1016/j.cplett.2023.140372

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The development of an efficient and stable hydrogen evolution reaction (HER) electrocatalyst is essential for industrial water splitting. Here, we used waste durian shells, cheap urea and palladium acetate to synthesize PdO supported nitrogen-doped biomass based carbon nanomaterials. The prepared Pd-N-CDS electrocatalyzed the hydrogen evolution reaction in 0.5 M H2SO4, and the overpotential recorded was 143 mV at 10 mA cm-2. In particular, the potential applied at a current density of 10 mA cm-2 obtained excellent stability using the chronoamperometry. In addition, the Pd oxide nanoparticles covered by the thin carbon layer cooperate to catalyze HER through the radiated electronic effect.

引用

页数：6

共 62 条

[1] Palladium Nanoparticle-Graphitic Carbon Nitride Porous Synergistic Catalyst for Hydrogen Evolution/Oxidation Reactions over a Broad Range of pH and Correlation of Its Catalytic Activity with Measured Hydrogen Binding Energy [J].

Bhowmik, Tanmay ;

Kundu, Manas Kumar ;

Barman, Sudip .

ACS CATALYSIS, 2016, 6 (03) :1929-1941

[2] Nanocomposites of 1D MoS2 with Polymer-Functionalized Nanotubes of Carbon and Borocarbonitride, and Their HER Activity [J].

Binwal, Devesh Chandra ;

Pramoda, K. ;

Zak, Alla ;

Kaur, Manjodh ;

Chithaiah, Pallellappa ;

Rao, C. N. R. .

ACS APPLIED ENERGY MATERIALS, 2021, 4 (03) :2339-2347

[3] Advanced Biomass-Derived Electrocatalysts for the Oxygen Reduction Reaction [J].

Borghei, Maryam ;

Lehtonen, Janika ;

Liu, Liang ;

Rojas, Orlando J. .

ADVANCED MATERIALS, 2018, 30 (24)

[4] Multiple Functional Biomass-Derived Activated Carbon Materials for Aqueous Supercapacitors, Lithium-Ion Capacitors and Lithium-Sulfur Batteries [J].

Chen, Kunfeng ;

Xue, Dongfeng .

CHINESE JOURNAL OF CHEMISTRY, 2017, 35 (06) :861-866

[5] Low-temperature and one-pot synthesis of sulfurized graphene nanosheets via in situ doping and their superior electrocatalytic activity for oxygen reduction reaction [J].

Chen, Yi ;

Li, Jing ;

Mei, Tao ;

Hu, Xian'gang ;

Liu, Dengwu ;

Wang, Juncheng ;

Hao, Ming ;

Li, Jinhua ;

Wang, Jianying ;

Wang, Xianbao .

JOURNAL OF MATERIALS CHEMISTRY A, 2014, 2 (48) :20714-20722

[6] Kinetic study of hydrogen evolution reaction on Ni30Mo70, Co30Mo70, Co30Ni70 and Co10Ni20Mo70 alloy electrodes [J].

Domínguez-Crespo, MA ;

Plata-Torres, M ;

Torres-Huerta, AM ;

Arce-Estrada, EM ;

Hallen-López, JM .

MATERIALS CHARACTERIZATION, 2005, 55 (01) :83-91

[7] Pd-Co2P nanoparticles supported on N-doped biomass-based carbon microsheet with excellent catalytic performance for hydrogen evolution from formic acid [J].

Duan, Jingmin ;

Xiang, Zhongqing ;

Zhang, Hongsong ;

Zhang, Bing ;

Xiang, Xu .

APPLIED SURFACE SCIENCE, 2020, 530

[8] Fe-Doped Ni3C Nanodots in N-Doped Carbon Nanosheets for Efficient Hydrogen-Evolution and Oxygen-Evolution Electrocatalysis [J].

Fan, Haosen ;

Yu, Hong ;

Zhang, Yufei ;

Zheng, Yun ;

Luo, Yubo ;

Dai, Zhengfei ;

Li, Bing ;

Zong, Yun ;

Yan, Qingyu .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2017, 56 (41) :12566-12570

[9] Nitrogen-doped porous activated carbon derived from cocoon silk as a highly efficient metal-free electrocatalyst for the oxygen reduction reaction [J].

Fu, Peng ;

Zhou, Lihua ;

Sun, Lihua ;

Huang, Baohua ;

Yuan, Yong .

RSC ADVANCES, 2017, 7 (22) :13383-13389

[10] Hierarchical molybdenum phosphide coupled with carbon as a whole pH-range electrocatalyst for hydrogen evolution reaction [J].

Ge, Riyue ;

Huo, Juanjuan ;

Liao, Ting ;

Liu, Yang ;

Zhu, Mingyuan ;

Li, Ying ;

Zhang, Jiujun ;

Li, Wenxian .

APPLIED CATALYSIS B-ENVIRONMENTAL, 2020, 260

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