Development of a Kinetic Model for the Direct Oxidation of Benzene to Phenol by Oxygen in Dielectric Barrier Discharge

被引：0

作者：

Ochered'ko, A. N. ^{[1
]}

Leshchik, A. V. ^{[1
]}

Kudryashov, S. V. ^{[1
]}

Ryabov, A. Yu. ^{[1
]}

机构：

[1] Russian Acad Sci, Siberian Branch, Inst Petr Chem, Tomsk 634055, Russia

来源：

HIGH ENERGY CHEMISTRY | 2023年 / 57卷 / 05期

关键词：

direct oxidation of benzene; phenol; dielectric barrier discharge; modeling; kinetics; CONVERSION; METHANE; ALKANES; PLASMA;

D O I：

10.1134/S0018143923050089

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

A simplified model of the process of benzene oxidation by oxygen in a dielectric barrier discharge has been developed. A kinetic scheme of oxidation is proposed that reflects the real chemistry of the process. The simulation results confirm the earlier assumptions about the main stages of the benzene oxidation process with oxygen.

引用

页码：436 / 439

页数：4

共 50 条

[31] Coupling of Dielectric Barrier Discharge and Cu-S-1 Catalyst for Direct Oxidation of Methane to Methanol [J].

Lv, Huan ;

Liu, Xinyuan ;

Hao, Yingzi ;

Yi, Yanhui .

PLASMA CHEMISTRY AND PLASMA PROCESSING, 2023, 43 (06) :1963-1978

[32] Direct Oxidation of Methane to Methanol Over Cu-Based Catalyst in an AC Dielectric Barrier Discharge [J].

Liang Huang ;

Xing-wang Zhang ;

Lin Chen ;

Le-cheng Lei .

Plasma Chemistry and Plasma Processing, 2011, 31 :67-77

[33] DIRECT SYNTHESIS OF PHENOL BY HYDROXYLATION OF BENZENE WITH OXYGEN AND HYDROGEN [J].

MIYAKE, T ;

HAMADA, M ;

SASAKI, Y ;

OGURI, M .

APPLIED CATALYSIS A-GENERAL, 1995, 131 (01) :33-42

[34] Features of Propylene Oxidation by Carbon Dioxide in Dielectric Barrier Discharge [J].

Ryabov, A. Yu ;

Kudryashov, S., V ;

Ochered'ko, A. N. .

HIGH ENERGY CHEMISTRY, 2022, 56 (03) :217-222

[35] Fluorescence measurement of atomic oxygen concentration in a dielectric barrier discharge [J].

Dvorak, P. ;

Mrkvickova, M. ;

Obrusnik, A. ;

Kratzer, J. ;

Dedina, J. ;

Prochazka, V. .

PLASMA SOURCES SCIENCE & TECHNOLOGY, 2017, 26 (06)

[36] Kinetic Analysis of Dielectric Layer Thickness on Nitric Oxide Removal by Dielectric Barrier Discharge [J].

Wang, Tao ;

Sun, Bao-min ;

Xiao, Hai-ping .

JAPANESE JOURNAL OF APPLIED PHYSICS, 2013, 52 (04)

[37] Removal of benzene as a tar model compound from a gas mixture using non-thermal plasma dielectric barrier discharge reactor [J].

Saleem, Faisal ;

Khoja, Asif Hussain ;

Umer, Jamal ;

Ahmad, Farhan ;

Abbas, Syed Zaheer ;

Zhang, Kui ;

Harvey, Adam .

JOURNAL OF THE ENERGY INSTITUTE, 2021, 96 :97-105

[38] Benzene transformation in two dielectric barrier discharge reactors having special arrangement [J].

Dey, Ghasiram .

PLASMA PROCESSES AND POLYMERS, 2019, 16 (12)

[39] Partial oxidation of n-pentane to syngas and oxygenates in a dielectric barrier discharge reactor [J].

Zhang, Xuming ;

Wenren, Yesheng ;

Chen, Jingqing ;

Zhang, Liancheng ;

Jin, Yuzhen ;

Liu, Zhen ;

Jin, Haozhe ;

Liu, Qi ;

Zhu, Zuchao .

FUEL, 2022, 307

[40] Hydrogen Production from Partial Oxidation of Methane by Dielectric Barrier Discharge Plasma Reforming [J].

Wang Hao ;

Song Ling-Jun ;

Li Xing-Hu ;

Yue Li-Meng .

ACTA PHYSICO-CHIMICA SINICA, 2015, 31 (07) :1406-1412

← 1 2 3 4 5 →