Environmental contamination characteristics of heavy metals from abandoned lead-zinc mine tailings in China

被引:16
作者
Han, Wei [1 ]
Zhao, Ruifeng [1 ]
Liu, Wanrong [1 ]
Wang, Yujing [1 ]
Zhang, Shuai [2 ]
Zhao, Kang [1 ]
Nie, Jinglei [1 ]
机构
[1] Minist Ecol & Environm, Solid Waste & Chem Management Ctr, Beijing, Peoples R China
[2] Zhejiang Univ, MOE Key Lab Soft Soils & Geoenvironm Engn, Hangzhou, Peoples R China
基金
国家重点研发计划;
关键词
heavy metals; lead-zinc mine; mine tailing; soil and groundwater; contamination; HEALTH-RISK; POLLUTION; SOILS; INDUSTRIAL; AREA;
D O I
10.3389/feart.2023.1082714
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
China holds large-scale lead-zinc mineral resources; however, mining activities often cause severe contamination by heavy metals. This study systemically assessed contamination by eight heavy metals (Cu, Zn, Cd, Pb, Cr, Hg, Ni, and As) in mine tailings, soil, and groundwater from 27 contaminated sites across China. Regarding mine tailings, 1% of the mine tailing samples were hazardous waste and 20% were class II non-hazardous waste. Regarding soil, Zn and Pb showed the highest mean concentrations, at 5574.67 mg/kg and 2034.88 mg/kg, respectively. The indexes of geo-accumulation (I-geo) of eight heavy metals ranged from -3.62 to 7.67, while Zn, Pb, and Cd showed the highest environmental risk levels as the priority pollutants. The contamination levels of these heavy metals in groundwater were generally in the order of Zn>As>Pb>Ni>Cd>Cu>Hg>Cr. In this study, 20% of the soil and 10% of the groundwater samples exceeded the corresponding quality limits. The content of heavy metals in soil, groundwater, and mine tailing were positively correlated, demonstrating the main pollution source and transport paths. The pollution levels of heavy metals in soil and groundwater were listed in the foremost and moderate positions compared with similar sites from other countries, respectively. These results may help determine the pollution levels of lead-zinc mining regions and direct the remediation activities of target sites to support the environmental management of abandoned mining and tailing waste in China.
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页数:9
相关论文
共 33 条
[1]   HEAVY-METAL POLLUTION IN JAMAICA .1. SURVEY OF CADMIUM, LEAD AND ZINC CONCENTRATIONS IN THE KINTYRE AND HOPE-FLAT DISTRICTS [J].
ANGLINBROWN, B ;
ARMOURBROWN, A ;
LALOR, GC .
ENVIRONMENTAL GEOCHEMISTRY AND HEALTH, 1995, 17 (02) :51-56
[2]   Environmental assessment of abandoned mine tailings in Adak, Vasterbotten district (northern Sweden) [J].
Bhattacharya, Aparajita ;
Routh, Joyanto ;
Jacks, Gunnar ;
Bhattacharya, Prosun ;
Morth, Magnus .
APPLIED GEOCHEMISTRY, 2006, 21 (10) :1760-1780
[3]   Land Use in Habitats Affects Metal Concentrations in Wild Lizards Around a Former Lead Mining Site [J].
Doya, Rio ;
Nakayama, Shouta M. M. ;
Nakata, Hokuto ;
Toyomaki, Haruya ;
Yabe, John ;
Muzandu, Kaampwe ;
Yohannes, Yared B. ;
Kataba, Andrew ;
Zyambo, Golden ;
Ogawa, Takahiro ;
Uchida, Yoshitaka ;
Ikenaka, Yoshinori ;
Ishizuka, Mayumi .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2020, 54 (22) :14474-14481
[4]   Comparison of Chemical Speciation of Lead, Arsenic, and Cadmium in Contaminated Soils from a Historical Mining Site: Implications for Different Mobilities of Heavy Metals [J].
Gankhurel, Baasansuren ;
Fukushi, Keisuke ;
Akehi, Akitoshi ;
Takahashi, Yoshio ;
Zhao, Xiaolan ;
Kawasaki, Kazuo .
ACS EARTH AND SPACE CHEMISTRY, 2020, 4 (07) :1064-1077
[5]   Lead, Zinc, Arsenic and Copper Pollution in the Alluvial Plain of a Mining Wadi: The Beal Case (Cartagena-La Union Mining District, SE Spain) [J].
Gonzalez-Fernandez, Oscar ;
Queralt, Ignacio ;
Carvalho, Maria Luisa ;
Garcia, Gregorio .
WATER AIR AND SOIL POLLUTION, 2011, 220 (1-4) :279-291
[6]  
Gunson AJ, 2001, Artisanal mining in the People's Republic of China
[7]   Mineralogy and chemical forms of lead and zinc in abandoned mine wastes and soils: An example from Morocco [J].
Iavazzo, Pietro ;
Adamo, Paola ;
Boni, Maria ;
Hillier, Stephen ;
Zampella, Mariavittoria .
JOURNAL OF GEOCHEMICAL EXPLORATION, 2012, 113 :56-67
[8]   Variations in heavy metal contamination of stream water and groundwater affected by an abandoned lead-zinc mine in Korea [J].
Lee, JY ;
Choi, JC ;
Lee, KK .
ENVIRONMENTAL GEOCHEMISTRY AND HEALTH, 2005, 27 (03) :237-257
[9]   A review of soil heavy metal pollution from mines in China: Pollution and health risk assessment [J].
Li, Zhiyuan ;
Ma, Zongwei ;
van der Kuijp, Tsering Jan ;
Yuan, Zengwei ;
Huang, Lei .
SCIENCE OF THE TOTAL ENVIRONMENT, 2014, 468 :843-853
[10]   Heavy metal concentration, potential ecological risk assessment and enzyme activity in soils affected by a lead-zinc tailing spill in Guangxi, China [J].
Liu, Kehui ;
Li, Chunming ;
Tang, Sanqi ;
Shang, Guiduo ;
Yu, Fangming ;
Li, Yi .
CHEMOSPHERE, 2020, 251