Recent Advances in Common Transition Metal-Based Single-Atom Nanozymes and Their Applications in Pollutant Detection and Degradation

被引:2
作者
Xie, Xiaoyi [1 ]
Zhang, Yi [2 ]
Li, Dong [2 ]
Fan, Yuxiu [1 ]
Huang, Bin [2 ]
Yang, Xiupei [1 ,2 ]
机构
[1] China West Normal Univ, Chem Synth & Pollut Control Key Lab Sichuan Prov, Nanchong 637009, Peoples R China
[2] Nanchong Food & Drug Inspect Inst, Nanchong 637000, Peoples R China
基金
中国国家自然科学基金;
关键词
pollutant degradation; pollutant detection; single-atom nanozymes; transition metal base; COLORIMETRIC DETECTION; CATALYSTS; NANOPARTICLES; PERFORMANCE;
D O I
10.1002/ppsc.202300039
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Nanozymes can be used as favorable substitutes for natural enzymes because of their strong catalytic activity and good stability. At the same time, research on single-atom catalysts (SACs) with isolated metal atoms as active centers is also in full swing, showing excellent performance in a variety of catalytic reactions. With the in-depth study of SACs, people have a comprehensive understanding of them and put forward the concept of single-atom nanozymes (SAzymes) by combining nanozymes with SACs. As a new type of nanomaterial, SAzymes have attracted great interest due to their remarkable catalytic activity and rapid energy conversion. However, most applications of SAzymes are mainly in the fields of biomedicine and biosensing, and less research has been done in the field of the environment. Based on the amazing ability of nanozymes to detect and degrade pollutants, SAzymes are also used in the environmental field, and even they will show better capabilities. This review mainly analyses common transition metal-based SAzymes and describes their applications in the field of environmental pollutants.
引用
收藏
页数:14
相关论文
共 103 条
[1]   Role of Nitrogen in Defect Evolution in Zinc Oxide: STEM-EELS Nanoscale Investigations [J].
Bazioti, Calliope ;
Azarov, Alexander ;
Johansen, Klaus M. ;
Svensson, Bengt G. ;
Vines, Lasse ;
Kuznetsov, Andrej Y. ;
Prytz, Oystein .
JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2019, 10 (16) :4725-4730
[2]   CuS and NiS Nanoparticle-Decorated Porous-Reduced Graphene Oxide Sheets as Efficient Peroxidase Nanozymes for Easy Colorimetric Detection of Hg(II) Ions in a Water Medium and Using a Paper Strip [J].
Borthakur, Priyakshree ;
Boruah, Purna Kanta ;
Das, Manash R. .
ACS SUSTAINABLE CHEMISTRY & ENGINEERING, 2021, 9 (39) :13245-13255
[3]   Multi-hierarchical profiling the structure-activity relationships of engineered nanomaterials at nano-bio interfaces [J].
Cai, Xiaoming ;
Dong, Jun ;
Liu, Jing ;
Zheng, Huizhen ;
Kaweeteerawat, Chitrada ;
Wang, Fangjun ;
Ji, Zhaoxia ;
Li, Ruibin .
NATURE COMMUNICATIONS, 2018, 9
[4]   Single-Atom Pd Nanozyme for Ferroptosis-Boosted Mild-Temperature Photothermal Therapy [J].
Chang, Mengyu ;
Hou, Zhiyao ;
Wang, Man ;
Yang, Chunzheng ;
Wang, Ruifeng ;
Li, Fang ;
Liu, Donglian ;
Peng, Tieli ;
Li, Chunxia ;
Lin, Jun .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2021, 60 (23) :12971-12979
[5]   Atomically dispersed Fe/Bi dual active sites single-atom nanozymes for cascade catalysis and peroxymonosulfate activation to degrade dyes [J].
Chen, Qiumeng ;
Liu, Yuan ;
Lu, Yuwan ;
Hou, Yuejie ;
Zhang, Xiaodan ;
Shi, Wenbing ;
Huang, Yuming .
JOURNAL OF HAZARDOUS MATERIALS, 2022, 422
[6]   Dual-active-site Fe/Cu single-atom nanozymes with multifunctional specific peroxidase-like properties for S 2-detection and dye degradation [J].
Chen, Xiaofang ;
Wang, Ya ;
Feng, Min ;
Deng, Die ;
Xie, Xiaoyi ;
Deng, Caixia ;
Khattak, Kashif Nawaz ;
Yang, Xiupei .
CHINESE CHEMICAL LETTERS, 2023, 34 (06)
[7]   Fe single atoms anchored on fluorine-doped ultrathin carbon nanosheets for sensitive colorimetric detection of p-phenylenediamine [J].
Chen, Xiaofang ;
Feng, Min ;
Xie, Xiaoyi ;
Zhang, Yi ;
Zhang, Jie ;
Yang, Xiupei .
TALANTA, 2022, 246
[8]   Atomically Dispersed Cu Nanozyme with Intensive Ascorbate Peroxidase Mimic Activity Capable of Alleviating ROS-Mediated Oxidation Damage [J].
Chen, Yuan ;
Zou, Hang ;
Yan, Bo ;
Wu, Xiaoju ;
Cao, Weiwei ;
Qian, Yihang ;
Zheng, Lei ;
Yang, Guowei .
ADVANCED SCIENCE, 2022, 9 (05)
[9]   Thermal Atomization of Platinum Nanoparticles into Single Atoms: An Effective Strategy for Engineering High-Performance Nanozymes [J].
Chen, Yuanjun ;
Wang, Peixia ;
Hao, Haigang ;
Hong, Juanji ;
Li, Haijing ;
Ji, Shufang ;
Li, Ang ;
Gao, Rui ;
Dong, Juncai ;
Han, Xiaodong ;
Liang, Minmin ;
Wang, Dingsheng ;
Li, Yadong .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2021, 143 (44) :18643-18651
[10]   Single-Atom Nanozyme Based on Nanoengineered Fe-N-C Catalyst with Superior Peroxidase-Like Activity for Ultrasensitive Bioassays [J].
Cheng, Nan ;
Li, Jin-Cheng ;
Liu, Dong ;
Lin, Yuehe ;
Du, Dan .
SMALL, 2019, 15 (48)