Experimental Study on the Effect of H2 on the Degradation of SF6 by Pulsed Dielectric Barrier Discharge

被引:6
作者
Li, Yalong [1 ]
Yang, Zhaodi [1 ]
Wang, Yufei [2 ]
Zhang, Xiaoxing [1 ]
Wan, Kun [1 ]
Zhang, Ying [3 ]
机构
[1] Hubei Univ Technol, Hubei Engn Res Ctr Safety Monitoring New Energy &, Wuhan 430068, Peoples R China
[2] State Grid Hubei Direct Current Co, Yichang 443002, Peoples R China
[3] Guizhou Power Grid Co Ltd, Sci Res Inst Elect Power, Guiyang 550002, Peoples R China
关键词
Degradation products; destruction and removal efficiency (DRE); dielectric barrier discharge (DBD); H-2; SF6; SULFUR-HEXAFLUORIDE; CO2; HYDROGENATION; DECOMPOSITION; ABATEMENT;
D O I
10.1109/TDEI.2023.3301828
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
Sulfur hexafluoride (SF6) is widely used in high-voltage gas insulation equipment, but SF6 has a strong greenhouse effect, with the "peak carbon dioxide emissions and carbon neutrality" goal proposed, its harmless degradation treatment has become an urgent problem in the power industry. In this article, it is proposed that SF6 degradation under H-2 synergy is based on pulsed dielectric barrier discharge (DBD) plasma technology. The results show that H-2 can significantly promote the degradation of SF6 and improve its destruction and removal efficiency (DRE). Among them, as the H-2 concentration increased gradually from 0.2% to 2%, the DRE of SF6 gradually increase. The complete removal of SF6 was achieved by adding 2% H-2 at a flow rate of 50 mL/min of 2% SF6 gas mixture and a power input of 55 W. The detection and analysis of SF6 discharge degradation products showed that the main products were SO2, SOF2, SO2F2, SiF4, and OF2. The addition of H-2 will inhibit the formation of S-O-F gas products, and promote the formation of SO2 and S elements. With the increase of H-2 concentration, the rate of S element generation gradually accelerated, and the selectivity of SO2 in gas decomposition products reached more than 50% when H-2 concentration was high. The results of this study provide a direction for the efficient degradation and product regulation of SF6.
引用
收藏
页码:448 / 456
页数:9
相关论文
共 29 条
[1]  
Ahmad Raza T., 2022, Turkish Journal of Electrical Power and Energy Systems, V2, P94
[2]   Atmospheric Chemistry of (CF3)2CF-CN: A Replacement Compound for the Most Potent Industrial Greenhouse Gas, SF6 [J].
Andersen, Mads P. Sulbaek ;
Kyte, Mildrid ;
Andersen, Simone Thirstrup ;
Nielsen, Claus J. ;
Nielsen, Ole John .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2017, 51 (03) :1321-1329
[3]   Potential of adsorbents and membranes for SF6 capture and recovery: A review [J].
Chuah, Chong Yang ;
Lee, Yechan ;
Bae, Tae-Hyun .
CHEMICAL ENGINEERING JOURNAL, 2021, 404
[4]   SF6 catalytic degradation in a γ-Al2O3 packed bed plasma system: A combined experimental and theoretical study [J].
Cui, Zhaolun ;
Zhou, Chang ;
Jafarzadeh, Amin ;
Meng, Shengyan ;
Yi, Yanhui ;
Wang, Yufei ;
Zhang, Xiaoxing ;
Hao, Yanpeng ;
Li, Licheng ;
Bogaerts, Annemie .
HIGH VOLTAGE, 2022, 7 (06) :1048-1058
[5]   CO2 Hydrogenation in a Dielectric Barrier Discharge Plasma Revealed [J].
De Bie, Christophe ;
van Dijk, Jan ;
Bogaerts, Annemie .
JOURNAL OF PHYSICAL CHEMISTRY C, 2016, 120 (44) :25210-25224
[6]   Oxidative Fluorination of Selenium and Tellurium Compounds using a Thermally Stable Phosphonium SF5- Salt Accessible from SF6 [J].
Eder, Tobias ;
Buss, Florenz ;
Wilm, Lukas F. B. ;
Seidl, Michael ;
Podewitz, Maren ;
Dielmann, Fabian .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2022, 61 (42)
[7]   The Activation of Sulfur Hexafluoride at Highly Reduced Low-Coordinate Nickel Dinitrogen Complexes [J].
Holze, Patrick ;
Horn, Bettina ;
Limberg, Christian ;
Matlachowski, Corinna ;
Mebs, Stefan .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2014, 53 (10) :2750-2753
[8]   Investigating the low cost photodegradation performance against organic Pollutants using CeO2/MnO2/ polymer blend nanostructures [J].
Hussien, Huda Abdul Jalil ;
Kadhim, Raheem G. ;
Hashim, Ahmed .
OPTICAL AND QUANTUM ELECTRONICS, 2022, 54 (11)
[9]   Chlorobenzene Removal Using DBD Coupled with CuO/γ-Al2O3 Catalyst [J].
Jin, Xingpeng ;
Wang, Guicheng ;
Lian, Liping ;
Gao, Fan ;
Zhang, Renxi ;
Zhao, Weixuan ;
Hou, Jianyuan ;
Chen, Shanping ;
Zhang, Ruina .
APPLIED SCIENCES-BASEL, 2021, 11 (14)
[10]   Comprehensive process and environmental impact analysis of integrated DBD plasma steam methane reforming [J].
King, Benjamin ;
Patel, Darsh ;
Chen, Johnny Zhu ;
Drapanauskaite, Donata ;
Handler, Robert ;
Nozaki, Tomohiro ;
Baltrusaitis, Jonas .
FUEL, 2021, 304