Zeeman spectroscopy and crystal-field analysis of low symmetry centres in Nd3+ doped Y2SiO5

被引：3
作者：
Alizadeh, Y. [1 ,2 ]
Wells, J-p R. [1 ,2 ]
Reid, M. F. [1 ,2 ]
Ferrier, A. [3 ,4 ]
Goldner, P. [3 ]
机构：
[1] Univ Canterbury, Sch Phys & Chem Sci, PB4800, Christchurch 8140, New Zealand
[2] Dodd Walls Ctr Photon & Quantum Technol, Dunedin, New Zealand
[3] PSL Univ, Inst Rech Chim Paris, Chim Paris Tech, CNRS, F-75005 Paris, France
[4] Sorbonne Univ, Fac Sci & Ingn, UFR933, F-75005 Paris, France
来源：
JOURNAL OF PHYSICS-CONDENSED MATTER | 2023年 / 35卷 / 30期
关键词：
Zeeman spectroscopy; neodymium; Y2SiO5; crystal field modelling; correlation crystal field; GLOBAL OPTIMIZATION; TRANSITIONS; CLUSTERS; LEVEL; IONS;
D O I：
10.1088/1361-648X/acceed
中图分类号：
O469 [凝聚态物理学];
学科分类号：
070205 ;
摘要：
We report on infrared to visible Zeeman absorption spectroscopy and parameterised crystal-field modelling of Nd3+ centres in Y2SiO5 through the use of experimentally inferred crystal-field energy levels and Zeeman directional electronic g values. We demonstrate that good agreement between the calculated and experimental crystal-field energy levels as well as directional Zeeman g values along all three crystallographic axes can be obtained. Further, we demonstrate that the addition of correlation crystal field effects successfully account for discrepancies that arise between the calculated and experimental values relevant to the H-2 11/2
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页数：11
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