Topologically Porous Heterostructures for Photo/Photothermal Catalysis of Clean Energy Conversion

被引：4
作者：
Gao, Fan [1 ,2 ]
Wang, Xinqiang [1 ]
Cui, Wen-Gang [1 ]
Liu, Yanxia [1 ]
Yang, Yaxiong [1 ]
Sun, Wenping [3 ,4 ]
Chen, Jian [1 ]
Liu, Ping [2 ]
Pan, Hongge [1 ,3 ,4 ]
机构：
[1] Xian Technol Univ, Inst Sci & Technol New Energy, Xian 710021, Peoples R China
[2] Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350116, Peoples R China
[3] Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China
[4] Zhejiang Univ, Sch Mat Sci & Engn, Hangzhou 310027, Peoples R China
来源：
SMALL METHODS | 2023年 / 7卷 / 04期
关键词：
COx hydrogenation; H-2; production; photo; photothermal catalysis; topologically porous heterostructures; LAYERED DOUBLE HYDROXIDES; METAL-ORGANIC FRAMEWORKS; PHOTOCATALYTIC CO2 REDUCTION; BAND-GAP; HIGH-PERFORMANCE; ALLOY CATALYSTS; RECENT PROGRESS; EFFICIENT; WATER; MOF;
D O I：
10.1002/smtd.202201532
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
As a straightforward way to fix solar energy, photo/photothermal catalysis with semiconductor provides a promising way to settle the energy shortage and environmental crisis in many fields, especially in clean energy conversion. Topologically porous heterostructures (TPHs), featured with well-defined pores and mainly composed by the derivatives of some precursors with specific morphology, are a major part of hierarchical materials in photo/photothermal catalysis and provide a versatile platform to construct efficient photocatalysts for their enhanced light absorption, accelerated charges transfer, improved stability, and promoted mass transportation. Therefore, a comprehensive and timely review on the advantages and recent applications of the TPHs is of great importance to forecast the potential applications and research trend in the future. This review initially demonstrates the advantages of TPHs in photo/photothermal catalysis. Then the universal classifications and design strategies of TPHs are emphasized. Besides, the applications and mechanisms of photo/photothermal catalysis in hydrogen evolution from water splitting and COx hydrogenation over TPHs are carefully reviewed and highlighted. Finally, the challenges and perspectives of TPHs in photo/photothermal catalysis are also critically discussed.
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页数：27
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