Cellulose nanofiber membrane modified with functionalized MIL-101 for enhanced hydrogen separation

被引：7
作者：
Zhou, Yichen [1 ]
Hu, Zhirong [1 ]
Yu, Mengjiao [1 ]
Zhang, Lu [1 ]
Yao, Jianfeng [1 ]
机构：
[1] Nanjing Forestry Univ, Coll Chem Engn, Jiangsu Prov Key Lab Green Biomass Based Fuels &, Jiangsu Coinnovat Ctr Efficient Proc & Utilizat F, Nanjing 210037, Peoples R China
来源：
CELLULOSE | 2023年 / 30卷 / 01期
关键词：
MIL-101; TEMPO-oxidized cellulose nanofibers; Mixed matrix membrane; Hydrogen separation; METAL-ORGANIC FRAMEWORK; MIXED-MATRIX MEMBRANES; UIO-66-NH2; REMOVAL; FILLER; IONS;
D O I：
10.1007/s10570-022-04877-z
中图分类号：
TB3 [工程材料学]; TS [轻工业、手工业、生活服务业];
学科分类号：
0805 ; 080502 ; 0822 ;
摘要：
Mixed matrix membranes (MMMs) are expected to be strong competitors in gas separation membranes. Nevertheless, the poor interaction between fillers and matrix is a major restriction to prepare MMMs with a higher separation performance. In this work, MIL-101(Cr) was functionalized with - NH2, -COOH, and benzenesulfonic acid (-PhSO3H) group and these functionalized MIL-101 particles were embedded in cellulose nanofibers (CNFs) to form MMMs. The interaction effect of functionalized MIL-101 with CNFs on the separation performance was discussed. After the adjustment of MIL-101-NH2 loading, the resulting MIL-101-NH2/CNF membrane with 5 wt% loading exhibited enhanced H-2 permeance of similar to 2.56 x 10(-7) mol m(-2) s(-1) Pa-1 with H-2/CO2 ideal selectivity of similar to 21.9.
引用
收藏
页码：201 / 209
页数：9
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