Contribution of electron density to plasma decomposition rate of methane

被引:3
作者
Sun, Haonan [1 ]
Katayama, Kazunari [2 ]
Oya, Makoto [2 ]
机构
[1] Kyushu Univ, Interdisciplinary Grad Sch Engn Sci, 6-1 Kasuga Koen, Kasuga, Fukuoka 8168580, Japan
[2] Kyushu Univ, Fac Engn Sci, 6-1 Kasuga Koen, Kasuga, Fukuoka 8168580, Japan
关键词
Plasma decomposition; methane; electron density; TRITIATED METHANE; HELIUM; ITER;
D O I
10.1016/j.fusengdes.2023.113885
中图分类号
TL [原子能技术]; O571 [原子核物理学];
学科分类号
0827 ; 082701 ;
摘要
Hydrogen extraction from methane will be a common and useful technique in hydrogen production systems and fuel cycle systems of deuterium-tritium fusion reactors. Since tritium is a precious fuel, it needs to be extracted from impurity gases such as tritiated methane contained in the exhaust gas from the plasma vessel of a fusion reactor. An experimental work was conducted in this study to investigate the electron collision of methane decomposition reaction in helium plasma. A special attention was placed on the electron density distribution in a plasma chamber, and the dependence of the decomposition rate on the methane/helium ratio. The experimental results showed that methane decomposition rate and electron density tended to increase linearly with increasing RF power. This suggests that a strong dependence of electron collision on methane decomposition. Eventually, the dependence of methane decomposition rate on electron density, total pressure, and inlet methane concentration in a gas flow-type helium plasma reactor was successfully formulated. This study provides new sight for demonstrating the contribution of electron density in RF plasma assisted methane decomposition, and the summarized equation offers potential for reactor design on promising energy utilization.
引用
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页数:5
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共 12 条
  • [1] Dry Reforming of Methane under Mild Conditions Using Radio Frequency Plasma
    Devid, Edwin
    Zhang, Diyu
    Wang, Dongping
    Ronda-Lloret, Maria
    Huang, Qiang
    Rothenberg, Gadi
    Shiju, N. Raveendran
    Kleyn, Aart W.
    [J]. ENERGY TECHNOLOGY, 2020, 8 (05)
  • [2] The ITER tritium systems
    Glugla, M.
    Antipenkov, A.
    Beloglazov, S.
    Caldwell-Nlchols, C.
    Cristescu, I. R.
    Cristescu, I.
    Day, C.
    Doerr, L.
    Girard, J. -P.
    Tada, E.
    [J]. FUSION ENGINEERING AND DESIGN, 2007, 82 (5-14) : 472 - 487
  • [3] Direct Decomposition Processing of Tritiated Methane by Helium RF Plasma
    Katayama, Kazunari
    Fukada, Satoshi
    [J]. FUSION SCIENCE AND TECHNOLOGY, 2017, 71 (03) : 426 - 431
  • [4] DEMONSTRATION OF TRITIUM EXTRACTION FROM TRITIATED METHANE IN HELIUM BY UTILIZING PLASMA DECOMPOSITION
    Katayama, Kazunari
    Fukada, Satoshi
    Nishikawa, Masabumi
    [J]. FUSION SCIENCE AND TECHNOLOGY, 2011, 60 (04) : 1379 - 1382
  • [5] Direct decomposition of methane using helium RF plasma
    Katayama, Kazunari
    Fukada, Satoshi
    Nishikawa, Masabumi
    [J]. FUSION ENGINEERING AND DESIGN, 2010, 85 (7-9) : 1381 - 1385
  • [6] Decomposition of methane to hydrogen using nanosecond pulsed plasma reactor with different active volumes, voltages and frequencies
    Khalifeh, Omid
    Mosallanejad, Amin
    Taghvaei, Hamed
    Rahimpour, Mohammad Reza
    Shariati, Alireza
    [J]. APPLIED ENERGY, 2016, 169 : 585 - 596
  • [7] Atomic and Molecular Processes in Plasma Decomposition Method of Hydrocarbon Gas
    Oya, Makoto
    Ikeda, Ryosuke
    Katayama, Kazunari
    [J]. PLASMA AND FUSION RESEARCH, 2020, 15 (15):
  • [8] Operational Tritium Inventories in the EU-DEMO Fuel Cycle
    Schwenzer, J. C.
    Day, C.
    Giegerich, T.
    Santucci, A.
    [J]. FUSION SCIENCE AND TECHNOLOGY, 2022, 78 (08) : 664 - 675
  • [9] Kinetic roles of vibrational excitation in RF plasma assisted methane pyrolysis
    Sun, Jintao
    Chen, Qi
    [J]. JOURNAL OF ENERGY CHEMISTRY, 2019, 39 : 188 - 197
  • [10] Tritium fuel cycle in ITER and DEMO: Issues in handling large amount of fuel
    Tanabe, T.
    [J]. JOURNAL OF NUCLEAR MATERIALS, 2013, 438 : S19 - S26