Ligand-assisted formation of mesoporous Zn-N-C to realize superior catalytic activity in solvent-free CO2 cycloaddition reactions

被引：1

作者：

Zhou, Yan ^{[1
,2
]}

Lv, Shanshan ^{[2
]}

Feng, Mengmeng ^{[2
]}

Qian, Changjin ^{[2
]}

Liu, Shoujie ^{[1
]}

Chen, Zheng ^{[2
,3
]}

机构：

[1] Anhui Univ, Sch Mat Sci & Engn, Hefei 230601, Peoples R China

[2] Anhui Normal Univ, Coll Chem & Mat Sci, Key Lab Funct Mol Solids, Minist Educ, Wuhu 241002, Peoples R China

[3] Nanjing Univ, State Key Lab Coordinat Chem, Nanjing 210023, Peoples R China

来源：

CHEMICAL COMMUNICATIONS | 2024年 / 60卷 / 19期

关键词：

DOPED CARBON; EFFICIENT; PERFORMANCE; FRAMEWORK; SITES;

D O I：

10.1039/d4cc00171k

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Mesoporous nitrogen-doped carbon-anchored single atom Zn was synthesized through etching of ZIF-8 with 1,10-phenanthroline and subsequent pyrolysis based on the Kirkendall effect. The abundant pores and increased surface area promote CO2 adsorption and mass transfer, thus significantly improving the catalytic activity in solvent-free cycloaddition of epoxides with CO2.

引用

页码：2641 / 2644

页数：4

共 30 条

[1] Electrocatalytic synthesis of organic carbonates
Anastasiadou, Dimitra
Hensen, Emiel J. M.
Figueiredo, Marta C.
[J]. CHEMICAL COMMUNICATIONS, 2020, 56 (86) : 13082 - 13092
[2] Task-Specific Ionic Liquid Functionalized-MIL-101(Cr) as a Heterogeneous and Efficient Catalyst for the Cycloaddition of CO2 with Epoxides Under Solvent Free Conditions
Bahadori, Mehrnaz
Tangestaninejad, Shahram
Bertmer, Marko
Moghadam, Majid
Mirkhani, Valiollah
Mohammadpoor-Baltork, Iraj
Kardanpour, Reihaneh
Zadehahmadi, Farnaz
[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING, 2019, 7 (04) : 3962 - 3973
[3] Tandem catalysis: one-pot synthesis of cyclic organic carbonates from olefins and carbon dioxide
Calmanti, Roberto
Selva, Maurizio
Perosa, Alvise
[J]. GREEN CHEMISTRY, 2021, 23 (05) : 1921 - 1941
[4] Atomic iron on mesoporous N-doped carbon to achieve dehydrogenation reaction at room temperature
Chen, Zheng
Yang, Wenjuan
Wu, Yue
Zhang, Chao
Luo, Jun
Chen, Chen
Li, Yadong
[J]. NANO RESEARCH, 2020, 13 (11) : 3075 - 3081
[5] Hierarchically mesoporous imidazole-functionalized covalent triazine framework: An efficient metal- and halogen-free heterogeneous catalyst towards the cycloaddition of CO2 with epoxides
Dai, Weili
Li, Qing
Long, Jianfei
Mao, Pei
Xu, Yong
Yang, Lixia
Zou, Jianping
Luo, Xubiao
[J]. JOURNAL OF CO2 UTILIZATION, 2022, 62
[6] Single Ni sites distributed on N-doped carbon for selective hydrogenation of acetylene
Dai, Xinyao
Chen, Zheng
Yao, Tao
Zheng, Lirong
Lin, Yue
Liu, Wei
Ju, Huanxin
Zhu, Junfa
Hong, Xun
Wei, Shiqiang
Wu, Yuen
Li, Yadong
[J]. CHEMICAL COMMUNICATIONS, 2017, 53 (84) : 11568 - 11571
[7] The State of Research Regarding Ordered Mesoporous Materials in Batteries
Du, Guangyu
Xu, Yuxia
Zheng, Shasha
Xue, Huaiguo
Pang, Huan
[J]. SMALL, 2019, 15 (11)
[8] Engineering pore-size distribution of metal-loaded carbon catalysts by in situ cavitation for boosting electrochemical mass transfer
Du, Hong-Gang
Zhang, Xue-Feng
Ding, Li-Wen
Liu, Juan-Li
Yu, Li-Hong
Zhang, Xiao-Han
Dou, Yuhai
Cao, Li-Ming
Zhang, Jia
He, Chun-Ting
[J]. APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY, 2024, 342
[9] Facile synthesis of single-atom electrocatalysts with tailored carbon architectures via a polyelectrolyte brush-templated-growth approach
Fu, Zhinan
Wang, Lizhen
Zhang, Weijun
Tang, Xuan
Xia, Wenxin
Li, Jinxia
Wang, Kuanwen
Zhou, Lihui
Guo, Xuhong
Dai, Sheng
[J]. JOURNAL OF MATERIALS CHEMISTRY A, 2023, 11 (33) : 17533 - 17541
[10] Photoinduced synergistic catalysis on Zn single-atom-loaded hierarchical porous carbon for highly efficient CO2 cycloaddition conversion
Gong, Lin
Sun, Ji
Liu, Yousong
Yang, Guangcheng
[J]. JOURNAL OF MATERIALS CHEMISTRY A, 2021, 9 (38) : 21689 - 21694

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