Near-Infrared Light-Driven Photocatalysis with an Emphasis on Two-Photon Excitation: Concepts, Materials, and Applications

被引：83
作者：
Han, Chuang [1 ]
Kundu, Bidyut Kumar [2 ]
Liang, Yujun [1 ]
Sun, Yujie [2 ]
机构：
[1] China Univ Geosci, Fac Mat Sci & Chem, Wuhan 430074, Hubei, Peoples R China
[2] Univ Cincinnati, Dept Chem, Cincinnati, OH 45221 USA
来源：
ADVANCED MATERIALS | 2024年 / 36卷 / 05期
基金：
美国国家科学基金会;
关键词：
near-infrared light; photocatalysis; rational design; two-photon absorption; UP-CONVERSION; RUTHENIUM COMPLEXES; OPTICAL-PROPERTIES; FOSSIL-FUELS; ABSORPTION; PLASMON; DESIGN; EFFICIENT; SEMICONDUCTOR; RED;
D O I：
10.1002/adma.202307759
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
Efficient utilization of sunlight in photocatalysis is widely recognized as a promising solution for addressing the growing energy demand and environmental issues resulting from fossil fuel consumption. Recently, there have been significant developments in various near-infrared (NIR) light-harvesting systems for artificial photosynthesis and photocatalytic environmental remediation. This review provides an overview of the most recent advancements in the utilization of NIR light through the creation of novel nanostructured materials and molecular photosensitizers, as well as modulating strategies to enhance the photocatalytic processes. A special focus is given to the emerging two-photon excitation NIR photocatalysis. The unique features and limitations of different systems are critically evaluated. In particular, it highlights the advantages of utilizing NIR light and two-photon excitation compared to UV-visible irradiation and one-photon excitation. Ongoing challenges and potential solutions for the future exploration of NIR light-responsive materials are also discussed. This review article presents a comprehensive survey of the latest developments in near-infrared (NIR) light harvesting strategies, with a particular focus on the emerging field of two-photon excitation NIR photocatalysis. The emphasis is on the unique benefits offered by NIR light and two-photon excitation when compared to UV-visible irradiation and one-photon excitation.image
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页数：25
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