XUV ionization of the H2 molecule studied with attosecond angular streaking

被引:4
作者
Serov, Vladislav V. [1 ]
Kheifets, Anatoli S. [2 ]
机构
[1] Saratov NG Chernyshevskii State Univ, Gen Theoret & Comp Phys, Saratov 410012, Russia
[2] Australian Natl Univ, Res Sch Phys, Canberra, ACT 2601, Australia
基金
澳大利亚研究理事会;
关键词
molecules; photoionization; time delay; TIME-DELAY; PHOTOIONIZATION; INTERFERENCE; PULSES;
D O I
10.1088/1361-6455/acaa23
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We study orientation and two-center interference effects in attosecond time-resolved photoionization of the H-2 molecule. Time resolution of extreme-ultraviolet ionization of H-2 is gained through the phase retrieval capability of attosecond angular streaking demonstrated earlier by Kheifets et al (2022 Phys. Rev. A 106 033106). Once applied to H-2, this technique delivers an anisotropic phase and time delay which both depend sensitively on the molecular axis orientation. In addition, the photoelectron momentum distribution displays a very clear two-center interference pattern. When the interference formula of Walter and Briggs (1999 J. Phys. B 32 2487) is applied, an effective photoelectron momentum appears to be greater than the asymptotic momentum at the detector. This effect is explained by a molecular potential well surrounding the photoemission center.
引用
收藏
页数:10
相关论文
共 52 条
[1]   Attosecond photoionisation time delays reveal the anisotropy of the molecular potential in the recoil frame [J].
Ahmadi, H. ;
Plesiat, E. ;
Moioli, M. ;
Frassetto, F. ;
Poletto, L. ;
Decleva, P. ;
Schroeter, C. D. ;
Pfeifer, T. ;
Moshammer, R. ;
Palacios, A. ;
Martin, F. ;
Sansone, G. .
NATURE COMMUNICATIONS, 2022, 13 (01)
[2]   Probing molecular environment through photoemission delays [J].
Biswas, Shubhadeep ;
Foerg, Benjamin ;
Ortmann, Lisa ;
Schoetz, Johannes ;
Schweinberger, Wolfgang ;
Zimmermann, Tomas ;
Pi, Liangwen ;
Baykusheva, Denitsa ;
Masood, Hafiz A. ;
Liontos, Ioannis ;
Kamal, Amgad M. ;
Kling, Nora G. ;
Alharbi, Abdullah F. ;
Alharbi, Meshaal ;
Azzeer, Abdallah M. ;
Hartmann, Gregor ;
Woerner, Hans J. ;
Landsman, Alexandra S. ;
Kling, Matthias F. .
NATURE PHYSICS, 2020, 16 (07) :778-+
[3]   Attosecond coupled electron and nuclear dynamics in dissociative ionization of H2 [J].
Cattaneo, L. ;
Vos, J. ;
Bello, R. Y. ;
Palacios, A. ;
Heuser, S. ;
Pedrelli, L. ;
Lucchini, M. ;
Cirelli, C. ;
Martin, F. ;
Keller, U. .
NATURE PHYSICS, 2018, 14 (07) :733-+
[4]   INTERFERENCE IN PHOTO-IONIZATION OF MOLECULES [J].
COHEN, HD ;
FANO, U .
PHYSICAL REVIEW, 1966, 150 (01) :30-&
[5]   Methods for the measurement of the duration of high-harmonic pulses [J].
Constant, E ;
Taranukhin, VD ;
Stolow, A ;
Corkum, PB .
PHYSICAL REVIEW A, 1997, 56 (05) :3870-3878
[6]   Theory of attosecond delays in laser-assisted photoionization [J].
Dahlstrom, J. M. ;
Guenot, D. ;
Klunder, K. ;
Gisselbrecht, M. ;
Mauritsson, J. ;
L'Huillier, A. ;
Maquet, A. ;
Taieb, R. .
CHEMICAL PHYSICS, 2013, 414 :53-64
[7]   Introduction to attosecond delays in photoionization [J].
Dahlstrom, J. M. ;
L'Huillier, A. ;
Maquet, A. .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2012, 45 (18)
[8]  
Driver T., 2020, 51 ANN M APS DIVISIO
[9]   Tunable isolated attosecond X-ray pulses with gigawatt peak power from a free-electron laser [J].
Duris, Joseph ;
Li, Siqi ;
Driver, Taran ;
Champenois, Elio G. ;
MacArthur, James P. ;
Lutman, Alberto A. ;
Zhang, Zhen ;
Rosenberger, Philipp ;
Aldrich, Jeff W. ;
Coffee, Ryan ;
Coslovich, Giacomo ;
Decker, Franz-Josef ;
Glownia, James M. ;
Hartmann, Gregor ;
Helml, Wolfram ;
Kamalov, Andrei ;
Knurr, Jonas ;
Krzywinski, Jacek ;
Lin, Ming-Fu ;
Nantel, Megan ;
Natan, Adi ;
O'Neal, Jordan ;
Shivaram, Niranjan ;
Walter, Peter ;
Wang, Anna Li ;
Welch, James J. ;
Wolf, Thomas J. A. ;
Xu, Joseph Z. ;
Kling, Matthias F. ;
Bucksbaum, Philip H. ;
Zholents, Alexander ;
Huang, Zhirong ;
Cryan, James P. ;
Marinelli, Agostino ;
Marangos, Jon P. .
NATURE PHOTONICS, 2020, 14 (01) :30-+
[10]   Attosecond angular streaking [J].
Eckle, Petrissa ;
Smolarski, Mathias ;
Schlup, Philip ;
Biegert, Jens ;
Staudte, Andre ;
Schoeffler, Markus ;
Muller, Harm G. ;
Doerner, Reinhard ;
Keller, Ursula .
NATURE PHYSICS, 2008, 4 (07) :565-570