Thermochemical Valorization of Waste Plastic for Production of Synthetic Fuels, Fine Chemicals, and Carbon Nanotubes

被引:9
作者
Tang, Karen Yuanting [1 ,2 ]
Chan, Chui Yu [3 ]
Chai, Casandra Hui Teng [3 ]
Low, Beverly Qian Ling [3 ,4 ]
Toh, Zhong Yi [3 ]
Wong, Benjamin Weng Leong [3 ]
Heng, Jerry Zhi Xiong [3 ]
Li, Zibiao [1 ,3 ]
Lee, Chi-Lik Ken [1 ]
Loh, Xian Jun [1 ,3 ]
Wang, Chi-Hwa [2 ]
Ye, Enyi [1 ,3 ]
机构
[1] ASTAR, Inst Sustainabil Chem Energy & Environm ISCE2, Singapore 627833, Singapore
[2] Natl Univ Singapore NUS, Dept Chem & Biomol Engn, Singapore 117585, Singapore
[3] ASTAR, Inst Mat Res & Engn IMRE, Singapore 138634, Singapore
[4] Univ Cambridge, Yusuf Hamied Dept Chem, Cambridge CB2 1EW, England
关键词
plastic upcycling; thermochemical valorization; pyrolysis; synthetic fuels; fine chemicals; carbon nanotubes; HIGH-DENSITY POLYETHYLENE; LIFE-CYCLE ASSESSMENT; FLUIDIZED-BED PYROLYSIS; MUNICIPAL SOLID-WASTE; CONICAL SPOUTED BED; CATALYTIC PYROLYSIS; THERMAL-DEGRADATION; SUPERCRITICAL WATER; BIOFUEL PRODUCTION; CIRCULAR ECONOMY;
D O I
10.1021/acssuschemeng.3c06276
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Globally, approximately 300 million metric tonnes of plastic waste are generated annually, and over 90% of them are either disposed to the landfill or incinerated. Though there are commitments to reduce waste plastics, it has its limitations. In this review, the various types of thermochemical processes (pyrolysis, gasification, and hydrothermal liquefaction) used for plastic waste upcycling are first introduced. The production of synthetic fuel, fine chemicals, and carbon nanotubes through these processes are then discussed, with the effects of each factor scrutinized. Technical challenges of the production using plastic waste and how it can be overcome are then highlighted. Economical and environmental assessment of the processes are also analyzed to determine whether such processes are viable for upcycling of waste plastic, closing the carbon economy loop.
引用
收藏
页码:1769 / 1796
页数:28
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