Greenhouse gas emissions from wastewater treatment plants in China: Historical emissions and future mitigation potentials

被引:43
作者
Yang, Mengjie [1 ]
Peng, Man [1 ]
Wu, Dong [1 ]
Feng, Haoyuan [1 ]
Wang, Yixian [2 ]
Lv, Yongpeng [2 ]
Sun, Fengyun [3 ]
Sharma, Sanjib [4 ]
Che, Yue [1 ]
Yang, Kai [1 ,5 ]
机构
[1] East China Normal Univ, Shanghai Engn Res Ctr Biotransformat Organ Solid, Sch Ecol & Environm Sci, Shanghai Key Lab Urban Ecol Proc & Ecorestorat, Shanghai 200241, Peoples R China
[2] Shanghai Municipal Engn Design Inst Grp CO LTD, Shanghai 200092, Peoples R China
[3] Shanghai Normal Univ, Sch Environm & Geog Sci, Shanghai 200234, Peoples R China
[4] Penn State Univ, Earth & Environm Syst Inst, University Pk, PA 16802 USA
[5] Shanghai Inst Pollut Control & Ecol Secur, Shanghai 200092, Peoples R China
基金
国家重点研发计划; 中国国家自然科学基金;
关键词
Wastewater treatment plants; Greenhouse gas emissions; Mitigation measures; Mitigation potentials; China; METHANE EMISSIONS; RESOURCE RECOVERY; NITROUS-OXIDE; ENERGY; CARBON; REDUCTION;
D O I
10.1016/j.resconrec.2022.106794
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Accurate estimation of greenhouse gas (GHG) emissions characteristics and future mitigation potentials of China's wastewater treatment plants (WWTPs) is essential to propose suitable mitigation strategies. Here we employ the population-equivalent method recommended by the IPCC to analyze GHG emission characteristics and hotspots of China's WWTPs from 2005 to 2020 and assess the mitigation potentials by 2035. Results show that GHG emissions from China's WWTPs more than tripled from 13.34 Mt CO2-eq in 2005 to 30.95 Mt CO2-eq in 2020. Due to the differences in electricity consumption intensity, emission factors, and economic development level, there is significant spatial heterogeneity in the amount, structure, and intensity of emissions by province. Scenario analysis reveals that energy-saving improvement generates the largest mitigation potential (15%), followed by operational optimization (10%) and thermal energy recovery (10%), while chemical energy recovery (4%) and solar energy utilization (3%) contribute the least. Taking all mitigation measures, emissions can reduce by about 41% to 21.14 Mt CO2-eq in 2035. What's more, the mitigation effect of different decarbonization measures varies among provinces. Our results highlight the need for targeted policy in priority areas and regionspecific strategies.
引用
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页数:10
相关论文
共 68 条
[11]   Methane emission during municipal wastewater treatment [J].
Daelman, Matthijs R. J. ;
van Voorthuizen, Ellen M. ;
van Dongen, Udo G. J. M. ;
Volcke, Eveline I. P. ;
van Loosdrecht, Mark C. M. .
WATER RESEARCH, 2012, 46 (11) :3657-3670
[12]   Site-specific carbon footprints of Scandinavian wastewater treatment plants, using the life cycle assessment approach [J].
Delre, Antonio ;
ten Hoeve, Marieke ;
Scheutz, Charlotte .
JOURNAL OF CLEANER PRODUCTION, 2019, 211 :1001-1014
[13]   Estimates and Predictions of Methane Emissions from Wastewater in China from 2000 to 2020 [J].
Du, Mingxi ;
Zhu, Qiuan ;
Wang, Xiaoge ;
Li, Peng ;
Yang, Bin ;
Chen, Huai ;
Wang, Meng ;
Zhou, Xiaolu ;
Peng, Changhui .
EARTHS FUTURE, 2018, 6 (02) :252-263
[14]   Insights into Nitrous Oxide Mitigation Strategies in Wastewater Treatment and Challenges for Wider Implementation [J].
Duan, Haoran ;
Zhao, Yingfen ;
Koch, Konrad ;
Wells, George F. ;
Zheng, Min ;
Yuan, Zhiguo ;
Ye, Liu .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2021, 55 (11) :7208-7224
[15]   Recovery of Nitrous Oxide from Wastewater Treatment: Current Status and Perspectives [J].
Duan, Haoran ;
Zhao, Yingfen ;
Koch, Konrad ;
Wells, George F. ;
Weissbach, Max ;
Yuan, Zhiguo ;
Ye, Liu .
ACS ES&T WATER, 2021, 1 (02) :240-250
[16]   Mitigating nitrous oxide emissions at a full-scale wastewater treatment plant [J].
Duan, Haoran ;
van den Akker, Ben ;
Thwaites, Benjamin J. ;
Peng, Lai ;
Herman, Caroline ;
Pan, Yuting ;
Ni, Bing-Jie ;
Watt, Shane ;
Yuan, Zhiguo ;
Ye, Liu .
WATER RESEARCH, 2020, 185
[17]  
EPA, 2018, EM GEN RES INT DAT E
[18]   Challenges in carbon footprint evaluations of state-of-the-art municipal wastewater resource recovery facilities [J].
Farago, Maria ;
Damgaard, Anders ;
Rebsdorf, Morten ;
Nielsen, Per Henrik ;
Rygaard, Martin .
JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2022, 320
[19]   Mapping multiple water pollutants across China using the grey water footprint [J].
Feng, Haoyuan ;
Sun, Fengyun ;
Liu, Yaoyi ;
Zeng, Peng ;
Deng, Lingzhi ;
Che, Yue .
SCIENCE OF THE TOTAL ENVIRONMENT, 2021, 785
[20]   Quantitative assessment of energy and resource recovery in wastewater treatment plants based on plant-wide simulations [J].
Fernandez-Arevalo, T. ;
Lizarralde, I. ;
Fdz-Polanco, F. ;
Perez-Elvira, S. I. ;
Garrido, J. M. ;
Puig, S. ;
Poch, M. ;
Grau, P. ;
Ayesa, E. .
WATER RESEARCH, 2017, 118 :272-288