Influence of microstructure and thermoelectric properties on the power density of multi-walled carbon nanotube/metal oxide hybrid flexible thermoelectric generators

被引:7
作者
Nayak, Ramakrishna [1 ]
Shetty, Prakasha [2 ,7 ]
Selvakumar, M. [2 ]
Shivamurthy, B. [3 ]
Rao, Ashok [4 ]
Sriram, K. V. [1 ]
Murari, M. S. [5 ]
Kompa, Akshayakumar [6 ]
Shanubhogue, U. Deepika [6 ]
机构
[1] Manipal Acad Higher Educ, Manipal Inst Technol, Dept Humanities & Management, Manipal 576104, Karnataka, India
[2] Manipal Acad Higher Educ, Manipal Inst Technol, Dept Chem, Manipal 576104, Karnataka, India
[3] Manipal Acad Higher Educ, Manipal Inst Technol, Dept Mech & Ind Engn, Manipal 576104, Karnataka, India
[4] Manipal Acad Higher Educ, Manipal Inst Technol, Ctr Clean Energy, Dept Phys, Manipal 576104, Karnataka, India
[5] Mangalore Univ, DST PURSE Lab, Mangalagangothri 574199, Karnataka, India
[6] Manipal Acad Higher Educ, Manipal Inst Technol, Dept Phys, Manipal 576104, Karnataka, India
[7] Alva Inst Engn & Technol, Dept Chem, Moodbidri 574225, Karnataka, India
关键词
Thermoelectricity; Cellulose acetate propionate; CuO; NiO; MWCNT; HIGH-PERFORMANCE; THERMAL-CONDUCTIVITY; FACILE SYNTHESIS; THIN-FILMS; ENHANCEMENT; ZNO; NIO; THERMOPOWER; COMPOSITES; MOBILITY;
D O I
10.1016/j.ceramint.2023.09.275
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
The quest for a low-cost, flexible thermoelectric generator using eco-friendly metal oxide-based materials for low-temperature applications has motivated this work. The work compares the performance of aminefunctionalized multi-walled carbon nanotubes (MWCNT-NH2) and metal oxide nanoparticles (CuO, NiO, and Fe2O3) ink-based hybrid flexible thermoelectric generators. Study reveals that the thermoelectric performance of a flexible thermoelectric generator improves by fine-tuning the materials crystallite size, bandgap, carrier concentration, carrier mobility, resistivity, the Seebeck coefficient, and micro-porosity of the ink film, which could be materialized by using hybrid thermoelectric materials. Among the three fabricated devices, MWCNT-NH2/NiO hybrid flexible thermoelectric generator exhibits a maximum power output of 1.44 nW at Delta T= 100 degrees C. The maximum power density displayed by MWCNT-NH2/NiO hybrid device is 59.3 nW/cm2 at Delta T= 100 degrees C, which is 23.28% and 332.8% higher than that of MWCNT-NH2/CuO and MWCNT-NH2/Fe2O3-based devices, respectively. The performance of MWCNT-NH2/NiO is comparatively superior to some previously reported works.
引用
收藏
页码:39307 / 39328
页数:22
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