Visualizing Nanoscale Interlayer Magnetic Interactions and Unconventional Low-Frequency Behaviors in Ferromagnetic Multishelled Structures

被引:31
作者
Chen, Guanyu [1 ]
Zhang, Ruixuan [2 ,3 ]
Yuan, Mingyue [1 ]
Xue, Shuyan [1 ]
Liu, Yihao [1 ]
Li, Bangxin [1 ,4 ,5 ]
Luo, Kaicheng [1 ]
Lai, Yuxiang [6 ]
Zhang, Jincang [3 ]
Lv, Hualiang [2 ]
Che, Renchao [1 ,3 ]
机构
[1] Fudan Univ, Acad Engn & Technol, Lab Adv Mat, Shanghai Key Lab Mol Catalysis & Innovat Mat, Shanghai 200438, Peoples R China
[2] Fudan Univ, Inst Optoelect, Shanghai Frontiers Sci Res Base Intelligent Optoel, Shanghai 200433, Peoples R China
[3] Zhejiang Lab, Hangzhou 311100, Peoples R China
[4] Fudan Univ, Dept Chem, Shanghai 200438, Peoples R China
[5] Fudan Univ, Shanghai Key Lab Mol Catalysis & Innovat Mat, Shanghai 200438, Peoples R China
[6] Hainan Univ, Innovat Inst Ocean Mat Characterizat, Pico Electron Microscopy Ctr, Ctr Adv Studies Precis Instruments, Haikou 570228, Peoples R China
基金
中国国家自然科学基金;
关键词
interlayer magnetic interaction; low-frequency electromagnetic absorption; multishelled structure; stray field visualization; FIELD;
D O I
10.1002/adma.202313411
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Precise manipulation of van der Waals forces within 2D atomic layers allows for exact control over electron-phonon coupling, leading to the exceptional quantum properties. However, applying this technique to diverse structures such as 3D materials is challenging. Therefore, investigating new hierarchical structures and different interlayer forces is crucial for overcoming these limitations and discovering novel physical properties. In this work, a multishelled ferromagnetic material with controllable shell numbers is developed. By strategically regulating the magnetic interactions between these shells, the magnetic properties of each shell are fine-tuned. This approach reveals distinctive magnetic characteristics including regulated magnetic domain configurations and enhanced effective fields. The nanoscale magnetic interactions between the shells are observed and analyzed, which shed light on the modified magnetic properties of each shell, enhancing the understanding and control of ferromagnetic materials. The distinctive magnetic interaction significantly boosts electromagnetic absorption at low-frequency frequencies used by fifth-generation wireless devices, outperforming ferromagnetic materials without multilayer structures by several folds. The application of magnetic interactions in materials science reveals thrilling prospects for technological and electronic innovation. A multishelled ferromagnetic material with controllable shell numbers is presented. By strategically regulating the nanoscale intershell magnetic interactions, the magnetic properties of each shell are fine-tuned. This approach has revealed distinctive magnetic characteristics including regulated magnetic domain configurations and enhanced effective fields. The unique magnetic coupling markedly improves electromagnetic absorption for fifth-generation frequencies. image
引用
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页数:13
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