Detection of tritium using ultrafast laser-induced breakdown spectroscopy

被引:11
作者
Harilal, Sivanandan S. [1 ]
Shaik, Abdul K. [1 ]
Kautz, Elizabeth J. [1 ,2 ]
Devaraj, Arun [1 ]
Casella, Andrew M. [1 ]
Senor, David J. [1 ]
机构
[1] Pacific Northwest Natl Lab, Richland, WA 99354 USA
[2] North Carolina State Univ, Nucl Engn Dept, Raleigh, NC 27695 USA
关键词
HYDROGEN; DYNAMICS; PLASMA; PROBE;
D O I
10.1039/d3ja00439b
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
Detection of nuclear materials and their radioisotopes with rapid, and standoff capability in addition to no sample preparation requirement is crucial to nuclear nonproliferation, safeguards, and security. In this work, we demonstrate the first application of ultrafast laser-induced breakdown spectroscopy to detect tritium (3H) during depth profiling of neutron-irradiated Zircaloy-4 samples. Detection of protium, deuterium and tritium using ultrafast LIBS with rapid, and standoff capability in addition to no sample preparation requirement which are crucial to nuclear nonproliferation, safeguards, and security
引用
收藏
页码:699 / 703
页数:6
相关论文
共 30 条
[21]  
Kramida A., 2012, NIST ATOMIC SPECTRA, DOI [10.18434/T4W30F, DOI 10.18434/T4W30F]
[22]   Review of Laser-Induced Plasma, Its Mechanism, and Application to Quantitative Analysis of Hydrogen and Deuterium [J].
Kurniawan, Koo Hendrik ;
Tjia, May On ;
Kagawa, Kiichiro .
APPLIED SPECTROSCOPY REVIEWS, 2014, 49 (05) :323-434
[23]  
LaGraffe D., 2022, HDB SECURITY SCI, P795
[24]   NanoSIMS Imaging and Analysis in Materials Science [J].
Li, Kexue ;
Liu, Junliang ;
Grovenor, Chris R. M. ;
Moore, Katie L. .
ANNUAL REVIEW OF ANALYTICAL CHEMISTRY, VOL 13, 2020, 13 :273-292
[25]   Hydrogen in zirconium alloys: A review [J].
Motta, Arthur T. ;
Capolungo, Laurent ;
Chen, Long-Qing ;
Cinbiz, Mahmut Nedim ;
Daymond, Mark R. ;
Koss, Donald A. ;
Lacroix, Evrard ;
Pastore, Giovanni ;
Simon, Pierre-Clement A. ;
Tonks, Michael R. ;
Wirth, Brian D. ;
Zikry, Mohammed A. .
JOURNAL OF NUCLEAR MATERIALS, 2019, 518 :440-460
[26]   Pu-239/Pu-240 isotope ratios determined using high resolution emission spectroscopy in a laser-induced plasma [J].
Smith, CA ;
Martinez, MA ;
Veirs, DK ;
Cremers, DA .
SPECTROCHIMICA ACTA PART B-ATOMIC SPECTROSCOPY, 2002, 57 (05) :929-937
[27]   Stand-off nuclear reactor monitoring with neutron detectors for safeguards and non-proliferation applications [J].
van der Ende, B. M. ;
Li, L. ;
Godin, D. ;
Sur, B. .
NATURE COMMUNICATIONS, 2019, 10 (1)
[28]   Monitoring of tritium and impurities in the first wall of fusion devices using a LIBS based diagnostic [J].
van der Meiden, H. J. ;
Almaviva, S. ;
Butikova, J. ;
Dwivedi, V ;
Gasior, P. ;
Gromelski, W. ;
Hakola, A. ;
Jiang, X. ;
Jogi, I ;
Karhunen, J. ;
Kubkowska, M. ;
Laan, M. ;
Maddaluno, G. ;
Marin-Roldan, A. ;
Paris, P. ;
Piip, K. ;
Pisarcik, M. ;
Sergienko, G. ;
Veis, M. ;
Veis, P. ;
Brezinsek, S. .
NUCLEAR FUSION, 2021, 61 (12)
[29]   Lithium Isotope Measurement Using Laser-Induced Breakdown Spectroscopy and Chemometrics [J].
Wood, Jason C. ;
Shattan, Michael B. .
APPLIED SPECTROSCOPY, 2021, 75 (02) :199-207
[30]   Plasma characteristics and element analysis of steels from a nuclear power plant based on fiber-optic laser-induced breakdown spectroscopy [J].
Wu, Jian ;
Yu, Han ;
Qiu, Yan ;
Zhang, Zhi ;
Liu, Tao ;
Xue, Fei ;
Yu, Weiwei ;
Li, Xingwen ;
Qiu, Aici .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2019, 52 (01) :1DUMMMY