Preparation of a nanostructured CdTe@CdS core-shell/Si photodetector by two-step laser ablation in liquid

被引:8
作者
Abdalaah, Yamamah K. [1 ]
Mahmood, Olfat Ahmed [1 ]
Shaker, Suaad S. [2 ]
Ismail, Raid A. [2 ]
机构
[1] Univ Diyala, Coll Sci, Dept Phys, Diyala, Iraq
[2] Univ Technol Baghdad, Dept Appl Sci, Baghdad, Iraq
来源
JOURNAL OF OPTICS-INDIA | 2025年 / 54卷 / 03期
关键词
Core-shell; CdTe@CdS; Laser ablation; Liquid; Photodetector; OPTOELECTRONIC PROPERTIES; OXIDE NANOPARTICLES; OPTICAL-PROPERTIES; EFFICIENCY; FABRICATION;
D O I
10.1007/s12596-024-01720-5
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
In this study, CdTe@CdS core-shell nanoparticles (NPs) were synthesized by pulsed laser ablation in distilled water. X-ray diffraction results showed a crystalline core/shell type. UV-Vis measurements revealed that the optical band gap of CdTe@CdS NPs was 2.25 eV. Energy-dispersive X-ray mapping confirmed the formation of the CdTe@CdS core/shell. Transmission electron microscope studies revealed that the core size (CdTe) is 16 nm, and the shell thickness (CdS) is around 3 nm. The photoluminescence (PL) spectrum confirms the emission of a strong and broad peak at 506 nm. The current characteristics of the n-CdTe@CdS/p-Si heterojunction exhibited rectifying behavior with an ideality factor of 4.3. The spectral operating region of the fabricated photodetector ranged from visible to near-infrared, with a maximum responsivity of 0.901 A/W at 810 nm. The specific detectivity and external quantum efficiency of CdTe@CdS/Si were 4.5 x 1011 Jones and 1.1 x 102%, respectively, at a bias voltage of - 7.5 V.
引用
收藏
页码:700 / 711
页数:12
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