Determining adsorbent performance degradation in pressure swing adsorption using a deep learning algorithm and one-dimensional simulator

被引:3
作者
Son, Seongmin [1 ,2 ]
机构
[1] Kyungpook Natl Univ, Dept Smart Plant Engn, Sangju 37224, South Korea
[2] Kyungpook Natl Univ, Dept Convergence & Fus Syst Engn, Sangju 37224, South Korea
关键词
Pressure Swing Adsorption; Degradation; Abnormal Detection; Simulation; METHANOL DEHYDRATION; DIMETHYL ETHER; MECHANISM; CATALYST; KINETICS; CHEMISTRY; STEP; TOOL;
D O I
10.1007/s11814-023-1524-x
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
This study proposes a methodology for diagnosing the degree of performance degradation of the adsorbent in pressure swing adsorption (PSA) plants using a one-dimensional simulator and a time-series deep learning algorithm. First, a 1D PSA simulator was developed using mathematical models and validated with previously published experimental data. The behavior change of the PSA plant according to the performance degradation was trained using a deep learning algorithm based on the developed simulator. The model combines the 1D convolutional neural network and long-short-term memory (LSTM) network. The prediction of the degradation degree of the internal adsorbent was then presented using a pretrained neural network. The developed methodology demonstrates a mean squared error lower than 10-6 when predicting the degree of adsorbent degradation from the adsorption-bed-temperature time-series profiles with an example. The methodology can be used to predictive maintenance strategy by identifying PSA performance degradation in real time without stopping operation.
引用
收藏
页码:2602 / 2611
页数:10
相关论文
共 41 条
[1]   Kinetic modeling of dimethyl ether synthesis in a single step on a CuO-ZnO-Al2O3/γ-Al2O3 catalyst [J].
Aguayo, Andres T. ;
Erena, Javier ;
Mier, Diana ;
Arandes, Jose M. ;
Olazar, Martin ;
Bilbao, Javier .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2007, 46 (17) :5522-5530
[2]   Development of Heterogeneous Catalysts for Dehydration of Methanol to Dimethyl Ether: A Review [J].
Bateni, Hamed ;
Able, Chad .
CATALYSIS IN INDUSTRY, 2019, 11 (01) :7-33
[3]   Understanding the interplay of bifunctional and electronic effects: Microkinetic modeling of the CO electro-oxidation reaction [J].
Baz, Adam ;
Holewinski, Adam .
JOURNAL OF CATALYSIS, 2020, 384 :1-13
[4]   DENSITY-FUNCTIONAL THEORY CALCULATIONS OF THE ACTIVATION OF METHANOL BY A BRONSTED ZEOLITIC PROTON [J].
BLASZKOWSKI, SR ;
VANSANTEN, RA .
JOURNAL OF PHYSICAL CHEMISTRY, 1995, 99 (30) :11728-11738
[5]   The mechanism of dimethyl ether formation from methanol catalyzed by zeolitic protons [J].
Blaszkowski, SR ;
vanSanten, RA .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1996, 118 (21) :5152-5153
[6]   Methanol Conversion to Dimethyl Ether in Catalytic Zeolite Membrane Reactors [J].
Brunetti, Adele ;
Migliori, Massimo ;
Cozza, Daniela ;
Catizzone, Enrico ;
Giordano, Girolamo ;
Barbieri, Giuseppe .
ACS SUSTAINABLE CHEMISTRY & ENGINEERING, 2020, 8 (28) :10471-10479
[7]   The Degree of Rate Control: A Powerful Tool for Catalysis Research [J].
Campbell, Charles T. .
ACS CATALYSIS, 2017, 7 (04) :2770-2779
[8]   Micro- and macro-kinetics: their relationship in heterogeneous catalysis [J].
Campbell, Charles T. .
TOPICS IN CATALYSIS, 1994, 1 (3-4) :353-366
[9]   Finding the rate-determining step in a mechanism - Comparing DeDonder relations with the "degree of rate control" [J].
Campbell, CT .
JOURNAL OF CATALYSIS, 2001, 204 (02) :520-524
[10]   Catalytic consequences of acid strength in the conversion of methanol to dimethyl ether [J].
Carr, Robert T. ;
Neurock, Matthew ;
Iglesia, Enrique .
JOURNAL OF CATALYSIS, 2011, 278 (01) :78-93